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Source-less density measurement using an adaptive neutron-induced gamma correction method

NUCLEAR ELECTRONICS AND INSTRUMENTATION

Source-less density measurement using an adaptive neutron-induced gamma correction method

Qiong Zhang
Yi Ge
Yu-Lian Li
Nuclear Science and TechniquesVol.34, No.8Article number 125Published in print Aug 2023Available online 28 Aug 2023
385011

The use of radioactive isotopes, such as Cs-137, to measure formation density is a common practice; however, it poses high risks such as environmental contamination from lost sources. To address these challenges, the use of pulsed neutron sources for density measurements, also known as "source-less density", has emerged as a promising alternative. By collecting gamma counts at different time gates according to the duty cycle of the pulsed sequence, the inelastic gamma component can be isolated to obtain more accurate density measurements. However, the collection of gamma rays during the neutron burst-on period often contains a proportion of capture gamma rays, which can reduce the accuracy of density measurements. This proportion can vary depending on the formation environment and neutron duty cycle. To address these challenges, an adaptive capture gamma correction method was developed for density measurements. This method distinguishes between "burst-on" and "burst-off" periods based on the gamma time spectra, and derives the capture ratio in the burst-on period by iteratively fitting the capture gamma time spectra, resulting in a more accurate net inelastic gamma. This method identifies the end of the pulse by automatically calculating the differential, and fits the capture gamma time spectra using Gaussian process regression, which considers the differences in formation attenuation caused by different environments. The method was verified through simulations with errors of below 0.025 g/cm3, demonstrating its adaptability and feasibility for use in formation density measurements. Overall, the proposed method has the potential to minimize the risks associated with radioactive isotopes and improve the accuracy of density measurements in various duty cycles and formation environments.

Neutron-induced gammaAdaptive correctionSource-less density
1

Introduction

The density of formation is a critical property that plays an indispensable role in reservoir evaluation [1, 2]. Traditionally, the chemical source Cs-137 has been used in nuclear well logging to measure the formation density [3]. However, the use of this source presents significant risks, including radiation hazards to field workers and potential environmental pollution if the source is lost [1]. To address these issues, the use of safer, controllable sources such as X-ray tubes and pulsed neutron generators has increased in the field [4-9]. Pulsed neutron generators are particularly effective in complicated wells because they emit high-energy neutrons that interact with the formation to generate secondary gamma rays with higher energies than those generated by Cs-137 sources, as shown in Fig. 1. In addition, high-energy neutrons emitted by pulsed neutron generators have good monochromaticity and extensive research exists on them. Pulsed neutron logging has been extensively researched, with established methods including measuring sigma, porosity, and elemental weight fractions based on thermal neutron time spectra or inelastic and capture gamma spectra [10-15]. However, density measurements using pulsed neutrons, also known as "source-less density measurement," presents a greater challenge, compared to chemical source density measurements [16]. These measurements are influenced by both neutron and gamma fields, resulting in a lower density sensitivity [17]. Currently, Schlumberger is the only company offering a commercially available source-less density tool. The initial field trials have been extremely well received [18-20].

Fig. 1
(Color online) Pulsed neutron measurement process. a. Pulsed neutron generator diagram. b. A single duty cycle in which the periodic generation of neutrons is controlled by electric pulses. c. Neutron-induced gamma produced in the formation during logging.
pic

In recent years, progress has been made in the field of source-less density measurements. Reichel et al. used a thermal neutron detector count to eliminate the influence of fast neutrons on the inelastic gamma count and calculated formation density [18]. Based on the fast-neutron gamma coupled field theory, Zhang et al. have quantified the influence of the formation parameters on the inelastic gamma-field distribution and proposed a density algorithm using the fast neutron count and near-to-far detector gamma count ratio [21]. Wang et al. use the high- and low-energy windows of net inelastic gamma spectra to improve the accuracy of the formation density by reducing the influence of pair production [22]. Zhang et al. develop a new source-less density measurement method using a boron sleeve gamma detector for high-brine oil and gas formations [23]. Dong et al. have treated the source-less density measurement as a regression problem and determine the net inelastic gamma ratio, fast neutron ratio, and borehole diameter from variables to calculate the density [24]. In addition to using inelastic gamma to measure the density, Zhang et al. compare and summarize three HI correction methods [25]. In these studies, the net inelastic gamma count ratio is directly used to calculate the density. In actual measurements, neutron-induced gamma rays are collected using time gates after neutron emission [18]. This means that during the neutron "burst-on" period, the collected gamma will inevitably contain some capture gamma rays; therefore, they must be corrected to obtain the net inelastic gamma, otherwise the accuracy of the density measurement will be affected.

The gamma collected during the burst-off" period (within a time gate of a few microseconds after neutron emission stops) can be approximately regarded as the capture gamma spectra. Therefore, if the capture gamma rays during the burst-on period can be calculated by matching the capture spectra during the burst-off period, net inelastic gamma counts can be obtained. Typically, the capture gamma is subtracted from the total gamma using a fixed proportional coefficient to obtain the net inelastic gamma count [26]. The methods for calculating fixed coefficients can be classified into two types: one is based on energy spectra only, and the other uses both energy and time spectra. Yuan et al. divided the gamma energy spectra into six energy ranges to obtain deduction coefficients and improved the accuracy of obtaining the concentration of elements by decomposing the inelastic gamma energy spectra [27]. Odom used a single exponential decay function to fit the time spectra for the capture gamma proportion [28], and Schmid and Li et al. use a double-exponential decay function to fit the time spectra to compensate for the borehole environment [29, 30].

Despite the availability of various methods for measuring the formation density, certain challenges remain unresolved. In real-world scenarios, the stability of the duty cycle varies according to the designated pulsed neutron tube. Furthermore, during downhole measurements, the environment changes according to the tool logs per vertical depth. Both challenges have significant effects on the capture gamma spectra. An example is shown in Fig. 2, where the capture gamma counts increase by 30.7% during the burst-on period when the duty cycle increases from 20% to 40%. The capture gamma counts decrease by 48% when the porosity increases from 0.9 p.u. to 20 p.u.

Fig. 2
Capture time spectra changes pertaining to the duty cycle (a) and formation porosity (b).
pic

Under such circumstances, previously reviewed methods can no longer prove efficient. This is because these methods employ a fixed decay function, such as the double exponential function, which cannot properly handle multiple changeable parameters, such as the duty cycle, and environmental factors, such as lithology, porosity, and borehole. This requires the manual adjustment of function-related parameters with respect to different duty cycles and environmental parameters, which hinders their ability to accurately capture gamma spectra.

To address these challenges, Gaussian process regression (GPR) was employed to develop an effective method for accurate neutron-induced gamma measurements [31]. This is caused by the following: (1) the kernel function in GPR provides an extremely strong fitting capability, which allows the time spectra obtained with different parameters to be adaptively matched, thus, overcoming the limitations of fixed functions. (2) GPR is suitable for small-sample fitting, making it ideal for fitting data points (small numbers) collected within a single pulse period. Typically, the actual time spectra are collected at time intervals of 1 and 100 µs as a pulse period, and data are acquired across multiple pulse periods to ensure the repeatability of the obtained time spectra. Consequently, the true sample data (average of the time spectra over multiple pulse periods) available for fitting are typically only 100 sample data points; thus, GPR can effectively handle such data. Using GPR to calculate the capture time spectra has the added benefit of providing probabilistic models, thus, enabling statistical error analysis for effective data quality control.

Fig. 3 provides an overview of the proposed method, which uses GPR to compensate for the impact of capture gamma rays during burst-on periods and obtain accurate formation densities. The proposed method comprises three main steps. First, the time spectra are matched based on the pulse characteristics to distinguish between burst-on and burst-off periods and adapt to different duty cycles. Second, GPR fits the gamma time spectra under burst-off periods to extract the capture gamma time spectra more accurately. Finally, net inelastic gamma is obtained using the capture gamma time spectra. The rest of the paper is organized as follows: Section 2 provides a step-by-step discussion of the proposed method, which employs a GPR algorithm framework. Section 3, presents the verification results of the proposed method based on Monte Carlo modelling under different duty cycles and formation environments. Finally, the conclusions are presented in Sect. 4.

Fig. 3
(Color online) Overview of the neutron-induced capture gamma correction method
pic
2

Methodology

2.1
Neutron-induced gamma time spectra feature analysis
A.
Overview of neutron-induced gamma: capture versus inelastic

To separate the capture and inelastic gamma rays collected during the burst-off period, it is necessary to analyze both types of gamma rays generated by the reaction. This involves the interaction of 14 MeV fast neutrons emitted by the D-T pulsed neutron generator with the formation, resulting in the production of secondary gamma rays through inelastic scattering and radiative capture. Based on one-group diffusion theory, the flux distribution of fast neutrons ϕN(r) at r can be expressed as Eq. (1): ϕN(r)=S04πr2er/λs (1) where S0 denotes the neutron strength, λs denotes the neutron slowing-down length, and r denotes the distance from the pulsed neutron source.

The probability of inelastic collisions between fast neutrons and nuclides is determined by the inelastic scattering cross-section, which varies for different nuclides. Therefore, the source of secondary inelastic gamma rays in the formation can be described as a set of inelastic gamma sources of M nuclides, as shown in Eq. (2). S(r)=iMSi(r)=iMNiϕN(r)ine_i, (2) where Ni is the number of gammas produced by the ith nuclide under fast neutron collisions, and ine_i is the inelastic scattering cross-section of the ith nuclide.

Using the Lagrange median value theorem, the inelastic gammas ϕinγ(R) detected at R can be expressed as ϕinγ(R)=S0iMNiine_i4πReR[1/λsα(1/λsμρ)], (3) where α (0,1), is the proportional coefficient from Lagrange’s median value theorem,  ρ represents the bulk density of formation, and μ is the mass absorption coefficient.

According to the thermal neutron diffusion theory, the thermal neutron flux mainly originates from fast neutron slowing-down and thermal neutron diffusion. Therefore, the thermal neutron flux distribution is given by Eq. (4): ϕt(r)=S0Lt24πr(λs2Lt2)(er/λsrer/Ltr), (4)  where ϕt(r) refers to the thermal neutron flux, λs is the fast neutron slowing-down length, and Lt is the thermal neutron diffusion length.

Capture gamma rays are generated by thermal neutrons. Similar to the derivation of the inelastic gamma flux, the capture gamma flux can be expressed as ϕcapγ(R)=S0Lt2iMNicap_i4πR(λs2Lt2)(eR[1/λsα1(1/λsμρ)]eR[1/Ltα2(1/λsμρ)]), (5)  where cap_i is the capture cross section of the ith nuclide.

Inelastic and capture gamma rays are represented separately in logarithmic form. From Eqs. (3) and (5), the gamma flux is affected by both neutron and gamma attenuation. The gamma attenuation is primarily influenced by the formation density, whereas the neutron attenuation is mainly influenced by the formation porosity. Therefore, by converting the fluxes to detector counts, we can approximate the detector counts as a function of the porosity, density, and source distance, as shown in Eq. (6): lnNinγ(R,φ,ρ)=lnS0iMNiine_i4πR+f(φ)(R)RαμρlnNcapγ(R,φ,ρ)=lnS0Lt2iMNicap_i4πR(λs2Lt2)+f(φ)(1R)+g(φ)(2R)+μρR(α2α1) (6)  where f(φ),  g(φ) are functions related to porosity (based on the transformation of diffusion or slowing-down length).

Based on Eq. (6), the intercepts of the curves when gamma varies with porosity (or density) are different because the elemental composition of the rocks varies with the lithology. The results shown in Fig. 4 are derived from the simulation results of the pulsed neutron tool presented in Section 3. With decreasing density (increasing porosity), the detector counts increase exponentially, matching the gamma attenuation trend. Fig. 4(b) shows that the trend of capture gamma rays with porosity is essentially the same for different lithologies (only the intercept is different). This indicates that neutron decay is dominant for the capture gamma. To summarize,1) neutron-induced gamma is affected by formation density, porosity, and lithology; 2) inelastic gamma is used for the measurement of formation density, whereas capture gamma reduces the sensitivity to formation density.

Fig. 4
(Color online) Inelastic and capture gamma changes with increasing porosity.
pic
B.
Time gate impact analysis

After analyzing the properties of the secondary gamma rays, it is necessary to investigate the composition of the capture and inelastic time spectra in the total time spectra. Owing to the periodic and repetitive nature of pulsed neutron sources, the following discussion is performed within a single-pulse period, as shown in Fig. 5.

Fig. 5
(Color online) The duty cycle of the pulse sequence. TOT (total) time gate corresponds to the burst-on period and CAP (total) time gate corresponds to the time when only captures occur. tburst corresponds to the duty cycle of the pulse neutron tube, tc is related to the tool setting, and tend is the end time of a pulse cycle, i.e., 100 μs.
pic

From Fig. 5, the count collected according to the actual count can be expressed as NTG_TOTγ=t=0tburstTS(t)NTG_CAPγ=t=tburst+tctendTS(t), (7) where TS refers to the time spectra (µs), NTG_TOTγ is the gamma count in the burst-on period, and NTG_CAPγ is the (capture) gamma count in the burst-off period.

Because the inelastic gamma rays generated after the burst-on period decrease to zero, the composition of the time spectra can be expressed as TS(t)=Ninγ(t)+Ncapγ(t)=Ninγ(t)+Ncapγ(t)(ttburst)Ncapγ(t)(t>tburst), (8) where Ninγ(t), Ncapγ(t) are the detector counts of inelastic and capture gamma rays at time t, respectively.

Gamma time spectra during the burst-on and burst-off periods are derived separately to analyze the time gate impact on the capture and inelastic gamma. Suppose that fast neutrons are emitted uniformly during the burst-on period; that is, k×t fast neutrons are generated. Therefore, the relationship between gamma and time during the burst-on time gate can be expressed as lnNinγ(t)=k(f(φ)(R)Rαμρ+c1)lnNcapγ(t)=kt(f(φ)(1R)+g(φ)(2R)ttburst                   +μρR(α2α1)+c2), (9) where c1=lnS0iMNiine_i4πR, c2=lnS0Lt2iMNicap_i4πR(λs2Lt2).

For the burst-off period, the time spectra can be approximated as the capture spectra based on Eq. (10): lnNinγ(t)0lnNcapγ(t)=lnNcapγ(tburst)R[Σvtα1(Σvtμρ)]t>tburst, (10) where Σ represents the macroscopic cross section and v is the neutron velocity.

Eqs. (8) and (9) show that the capture gamma collected in the TOT time gate increases with an increase in the burst time. Fig. 6 shows an example of the simulation results obtained during the burst-on period under different duty cycles. The total counts during the burst-on period decreased with increasing porosity, which corresponded to increasing hydrogen content, indicating that neutron attenuation played a dominant role. During the burst-on period, the percentage of capture gamma rays increased with an increasing duty cycle, whereas with an increase in porosity, the proportion of capture gamma rays decreased. This demonstrates that the capture spectra parameters vary with changes in the duty cycle and environmental parameters.

Fig. 6
Effect of different duty cycles on the TOT time gate: a. Total counts under different duty cycles. The vertical coordinate refers to the logarithm of the counts. b. Proportion of capture gamma in the TOT time gate.
pic

In conclusion, the correction of the capture gamma contributes to obtaining counts where gamma attenuation dominates, thus, improving the sensitivity of source-less density measurements to formations. Considering that the capture gamma is related to the duty cycle and environmental parameters during the burst-on period, an adaptive capture correction method is designed. This method is discussed in Sect. 2.2.

2.2
Burst-on period count optimization
A.
Data pre-processing

The distribution of neutrons emitted by a pulsed neutron generator may be shaped differently than that controlled by electrical pulses, owing to hardware constraints. Therefore, it is necessary to first identify the pulse shape, that is, the end time (tburst) of the burst-on period. Because no new fast neutrons are emitted during the burst-off period, the count of the time spectra collected after the burst-on period is significantly lower than that in the burst-on period; that is, the function TS(t) is discontinuous and varies significantly at the end of the burst-on period. Therefore, the end time of the burst period can be determined by using an enumeration algorithm that compares the counts of adjacent samples within a pulse period, as shown in Eq. (11). Subsequently, the pulse shape can be matched and the time spectra can be divided, as shown in Fig. 7. tburst=argmaxtTS(t)t, t=1, 2, , 100 μs (11)  where TS denotes the time spectra and t denotes time (μs).

Fig. 7
(Color online) Data collection and preprocessing. FM: Formation environment parameter, D: duty cycle.
pic
B.
Capture gamma time spectra derivation

By identifying the width of the burst period tburst, the time spectra of the capture gamma rays within a pulse period can be extracted from the total time spectra. The capture-time spectra calculation process is shown in Fig. 8, and a detailed derivation is presented below.

Fig. 8
(Color online) Obtaining the capture spectra based on GPR. Using the time spectra within the CAP time gate, the capture data within tbursttc are calculated. One time point at a time is extrapolated to iteratively calculate the capture spectra under the burst-off period.
pic

As the capture spectra are continuous, it is assumed that the time spectra satisfy a Gaussian process. The time spectra within the TOT and CAP time gates are fitted using GPR. TS(Ton)GP([00],Kon),Ton=[0, , tburst]TS(Toff)GP([00],Koff),Toff=[tc, , tend], (12) where Ton and Toff are the time-sampling points within the TOT and CAP time gates, respectively, and Kon and Koff are the corresponding covariance matrices.

The time spectra obtained using the CAP time gate are expressed as TS(Toff)N([00],[k(tc,tc)k(tc,tend)k(tend,tc)k(tend,tend)]), (13)  k(ti,tj)=σTS2exp((titj)22l2), (14) where σTS2, l are the hyperparameters in k. The larger σTS2, the larger the variance.

Let θ=σTS, l, then the corresponding hyperparameters are solved by maximizing the likelihood function, as shown in the following equation: θ=argmaxθlogp(TS(Toff)|t,θ). (15)

After establishing the GPR model based on the time spectra in the CAP time gate according to the Eq. (15), the calculation of the capture gamma spectra at other time points can be expressed as Eq. (16) because the new time-point counts still obey the Gaussian distribution: [TS(T)TScapγ(T*)]N([μμ*],[K(T,T)K(T,T*)K(T*,T)K(T*,T*)]), (16) where T*[tburst, tburst+tc), TToff.

The calculated distribution of the capture gamma rays in the burst-off period is given by TScapγ(T*)N(μ*, Σ*), (17)  where μ*=K(T*, T)(K(T, T)+σ2)1TS(T),Σ*=K(T*, T*)+ σ2 K(T*, T)(K(T, T)+σ2)1K(T, T*). (18) 

To further illustrate these steps, the simulation results with a duty cycle of 30% is used as an example. Fig. 9 shows the calculation of the capture gamma rays during the burst-off period, using the total time spectra as the input. The true capture spectra (obtained by Geant4 physical process identification) are shown in blue, and the calculated results are shown in red. Capture spectra can be obtained after matching the burst-on periods in the same manner. After matching, the capture spectra within a single pulse period are obtained using Eq. (19): TScapγ*(t)=TSon(t)(TSon(tburst)TScapγ(tburst)),ttburstTScapγ(T*),t>tburst. (19)

Fig. 9
Comparison between calculated and true values of capture time spectra during the burst-off period.
pic

The capture counts at time point tburst are jointly determined with the calculated results under the burst-on and burst-off periods, thus, adjusting Eq. (17) again. The distribution of capture gamma rays over time is obtained using Eq. (19), as shown in Fig. 10.

Fig. 10
(Color online) Comparison of the calculated capture spectra to true capture and total time spectra per pulse cycle.
pic
C.
Density measurement

The inelastic gamma time spectra are obtained by subtracting the capture spectra from the total time spectra, that is, the net inelastic gamma count is obtained, as shown in Eq. (20). Because the capture spectra are derived from the total time spectra, the method can be adapted to different porosities and densities of the formation, as well as different duty cycles of the neutron source: Nninγ=t=0tburstTSineγ(t)=t=0tburst(TS(t)TScapγ*(t)), (20) where Nninγ is the net inelastic gamma obtained from the calculated inelastic time spectra TSineγ(t).

The algorithm below describes the calculation of the net inelastic gamma. This algorithm can be applied to both near and far source detectors to calculate the count ratio for the acquisition of the formation density.

Algorithm: Acquisition of adaptive net inelastic gamma
Input: total time spectra TS
Output: net inelastic gamma count ratio Nniny
Initialize t, tburst, LOSS
for t < 100 do
  Compute the loss function: LOSS = TS(t)t
  if LOSS is maximum value, then
      tburst=t
  end
end
for t=tc; t > tburst do
    Calculate burst-off capture gamma time spectra with GPR:TScapγ(T*)
    t = t-1
end
Match the burst-on time spectra TSon(T)
Calculate burst-on capture gamma time spectra: TSon(T)(TSon(tburst)TScapγ(tburst))
Calculate net inelastic gamma counts: Nninγ=t=0tburst(TS(t)TScapγ*(t))
Show more

For a single detector, formation density ρ is expressed as ρ=1Rαμ[lnS0iMNiin_i4πRR(1α)1/λslnϕinγ(R,φ,ρ)] (21)

For an established tool structure for source-less density measurements, that is, two gamma detectors and two thermal neutron detectors, to correct the influence of the hydrogen index on the density measurement, formulae. (21) can be further written as ρ=AlnNinγ1Ninγ2+BlnNn1Nn2+C, (22) where Ninγ1 and Ninγ2  are the counts of near and far gamma detectors after capture correction, respectively; Nn1 and Nn2 are counts of near and far neutron detectors, respectively; and A, B, and C are constant coefficients.

3

Verification using Monte Carlo modelling

Based on theoretical derivations, the pulsed neutron density logging is influenced by formation parameters and the duty cycle of the pulsed neutron tube. To test the applicability and adaptiveness of the method, a dataset of 288 models with different parameters is simulated, as presented in Table 1. Because most pulsed-neutron density measurements use a 20% duty cycle while other pulsed neutron applications use a 30% duty cycle, 20%, 30%, and 40% are chosen to verify the adaptability of the method to the duty cycle (a significantly high duty cycle is not conducive to the collection of inelastic gamma rays). The source-less density tool has four sets of detectors, as shown in Fig. 11. Both gamma detectors are sodium iodide detectors, and the far and near neutron detectors consisted of two He3 tubes.

Table 1
Parameters of the simulation models.
Lithology Porosity (p.u.) Pore fluid Duty cycle Borehole diameter (mm)
Dolomite 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Limestone 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Sandstone 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Anhydrite 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Illite 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Kaolinite 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Montmorillonite 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Chlorite 0.9~40 Water, oil, gas 20%, 30%, 40% 216
Show more
Fig. 11
(Color online) Overview of the source-less density tool model. a. Schematic diagram of the tool structure. b. Geant4 simulation. c. Detector parameters.
pic

The simulation collects the time spectra of the gamma as an input, whereas pure inelastic gamma is collected as a reference through physical process identification. The method is validated in two progressive parts: detector count ratio and density calculations.

3.1
Calculation of the inelastic count ratio

Because the count ratio can minimize the effect of the in-well environment on the tool response and improve its sensitivity to formation, it is used in the calculation of the formation density, as shown in Eq. (22). Thus, the method is validated using detector count ratio Rγ as given Eq. (23): Rγ=Ninγ1Ninγ2. (23)  where Ninγ1 and Ninγ2 are near and far detector counts, respectively.

The statistical error of the count ratio obtained from the simulation can be calculated using Eq. (24): SE = 1Ninγ1+1Ninγ2×100% (24) where SE refers to a statistical error.

For the count ratios, the relative error is used to evaluate the calculated results expressed in Eq. (25). When the relative error between the calculated and simulation results is less than the statistical error of the simulation data, the calculated results satisfied the accuracy. RE = |PREMC|MC×100%, (25) where PRE is the calculated count ratio, MC is the simulated count ratio, and RE is the relative error.

The relative error between the calculated count ratio and the true value is less than the statistical error in 281 out of the 288 data points (97.6%), which indicates that the method can effectively correct the effect of capture. Part of the data that did not satisfy the error is related to the case where the duty cycle is 40% (the larger the duty cycle, the greater the impact of capture). To further test the applicability of the method, the results are discussed for three cases: the impact of 1) the duty cycle, 2) environmental parameters, and 3) multiparameter variation.

3.1.1
Case1: Duty cycle impact analysis

In this case, the formation lithology is limestone and the pores are filled with freshwater. The results obtained for the different duty cycles are presented in Table 2 and Fig. 12.

Table 2
Comparison results pertaining to different duty cycles under limestone.
Duty cycle (%) Porosity (p.u.) True count ratio Calculated count ratio Statistical error (%) Relative error (%)
20 0.9 66.71 65.63 4.01 1.62
  10 65.83 65.44 3.87 0.59
  20 58.53 57.35 3.91 2.02
  40 51.33 52.66 3.56 2.59
30 0.9 65.4 67.62 3.77 3.39
  10 64.55 65.11 3.66 0.87
  20 58.33 57.34 3.50 1.70
  40 53.28 53.89 3.66 1.14
40 0.9 65.92 67.22 3.79 1.97
  10 65.55 66.17 3.60 0.95
  20 57.33 56.21 3.57 1.95
  40 52.28 52.19 3.78 0.17
Show more
Fig. 12
Comparison between the detector count ratio and error at different duty cycles (limestone).
pic

As shown in Fig. 12, the net inelastic gamma count ratio decreases with increasing porosity. The trend of the net inelastic gamma count ratio with porosity is similar at different duty cycles, which indicates that the duty cycle does not affect the source-less density measurements using the inelastic gamma count ratio. Comparing the statistical error of the true ratio and the relative error, the relative errors of all the test data in limestone are less than the statistical errors, which shows that the proposed method can effectively deduce the capture under different duty cycles.

3.1.2
Case2: Environmental parameters impact
A.
Lithology variation

Because lithology has a large influence on gamma attenuation, particularly the capture gamma, the results obtained under eight different lithologies are compared in this case (except for dolomite and sandstone, which all belong to the mineral category). In this case, the duty cycle is 20%, and the pore fluid is water.

Secondary gamma production is correlated with the corresponding element (as shown in Eq. ((2))), the lithology has a strong influence on the detector count ratio. Table 3 and Fig. 13 present the results of the inelastic gamma compared with the capture-corrected inelastic gamma. In terms of relative errors, the errors are relatively higher for various types of minerals. For example, chlorite-containing iron also increases capture counts. These results illustrate that this method can also be applied to acquire net inelastic gamma under different lithologies.

Table 3
Comparison results for different lithology.
Lithology Porosity (p.u.) True count ratio Calculated count ratio Statistical error (%) Relative error (%)
Dolomite 0.9 85.4 84.62 3.01 0.91
  20 80.53 78.35 2.86 2.71
Sandstone 0.9 67.34 67.64 3.07 0.45
  20 60.45 62.09 2.96 2.71
Anhydrite 0.9 77.65 78.41 4.68 0.98
  20 65.89 65.63 4.39 0.39
Illite 0.9 88.65 91.39 4.49 3.09
  20 73.47 75.69 4.69 3.02
Kaolinite 0.9 77.44 74.67 4.84 3.58
  20 64.65 66.88 4.88 3.45
Montmorillonite 0.9 70.26 68.57 4.41 2.41
  20 65.27 63.25 4.53 3.09
chlorite 0.9 75.65 76.1 4.17 0.59
  20 66.76 64.17 4.29 3.88
Show more
Fig. 13
(Color online) Comparison of the detector count ratio and error for different lithology. The porosity is 0.9 p.u. in the left and 20 p.u. in the right figure.
pic
B.
Pore fluid variation

The formation fluids typically include oil, gas, and water. Among them, gas contains a much lower hydrogen index than oil and water, which affects the attenuation of neutrons at different porosities, thus, affecting the distribution of secondary gamma rays. This case is used to verify the adaptiveness of the capture-correction method under different pore fluids by varying the pore fluid type using dolomite and a 30% duty cycle (to avoid duplication of data). A comparison of the results is presented in Table 4 and Fig. 14. Because the gas density is the lowest, the gamma decay is the weakest at the same porosity. The hydrogen index of the gas is also the lowest, and the neutron attenuation is still the weakest. The final count ratios of the three pore fluids are shown in Fig. 14; the order of the detector count ratios under the same porosity is water > oil > gas. In addition, the count ratio under gas varied the most with porosity. Overall, the relative errors are less than the statistical errors of all the results, which indicates that the capture correction method can effectively correct the capture at different pore fluids.

Table 4
Comparison results for different pore fluids in dolomite.
Pore fluid Porosity (p.u.) True count ratio Calculated count ratio Statistical error (%) Relative error (%)
Oil 0.9 86.63 83.57 3.83 3.53
Oil 5 84.41 85.58 3.11 1.39
Oil 20 78.94 81.13 3.70 2.77
Oil 30 68.91 70.28 3.43 1.99
Oil 40 63.38 65.27 3.33 2.98
Gas 0.9 77.68 75.78 3.65 2.45
Gas 5 70.67 68.87 3.47 2.55
Gas 20 55.67 57.14 3.01 2.64
Gas 30 47.11 48.26 2.71 2.44
Gas 40 36.7 37.23 2.39 1.44
Water 0.9 88.4 86.62 3.37 2.01
Water 5 85.13 84.63 3.41 0.59
Water 20 81.42 80.35 3.67 1.31
Water 30 70.41 71.76 3.79 1.92
Water 40 62.13 61.1 3.56 1.66
Show more
Fig. 14
(Color online) Comparison between the detector count ratio and error for different pore fluids.
pic
3.1.3
Case3: Duty cycle, lithology, pore fluid variation

In this case, the duty cycle, lithology, and pore fluid are changed to further verify the accuracy of the net inelastic gamma count ratio obtained using the capture-gamma correction method. As shown in Fig. 15 and Table 5, the 12 sets of samples consisted of three duty cycles, five lithologies, and three pore fluids.

Table 5
Comparison results for different duty cycles and environment parameters.
Duty cycle (%) Lithology pore fluid Porosity (p.u.) True count ratio Calculated count ratio Statistical error (%) Relative error (%)
20 Sandstone Water 0.9 67.34 67.64 3.07 0.45
20 Sandstone Water 40 50.52 51.52 3.17 1.98
20 Kaolinite Gas 0.9 73.73 75.32 2.65 2.16
20 Kaolinite Gas 40 39.47 40.46 3.28 2.51
30 Limestone Gas 0.9 65.23 63.5 3.26 2.65
30 Limestone Gas 40 33.99 34.33 2.26 1.00
30 Illite Oil 0.9 83.86 84.15 2.45 0.35
30 Illite Oil 40 64.71 66.08 2.19 2.12
40 Sandstone Gas 0.9 60.43 60.9 3.11 0.78
40 Sandstone Gas 40 46.73 47.15 3.35 0.90
40 Dolomite Oil 0.9 81.3 82.3 4.20 1.23
40 Dolomite Oil 40 52.07 52.69 3.05 1.19
Show more
Fig. 15
(Color online) Comparison of the detector count ratio at different duty cycles and environment parameters.
pic

The results shown in Fig. 15, Track4, indicate that the proposed method can effectively adapt to different duty cycles and environmental parameters. Relative errors (orange line) are less than absolute errors (blue line), demonstrating the adaptability of the method. The following conclusions can be made:

• The duty cycle of the system directly affects the proportion of capture during the burst period. Moreover, increasing the duty cycle results in a higher proportion of capture; however, this can reduce the accuracy of subsequent formation density measurements.

• The lithology has a significant impact on the distribution of the secondary gamma field.

• Differences in pore fluids affect the neutron field distribution, causing an increased slowing of neutrons by the medium and reduced capture gamma rays reaching the detector.

3.2
Formation density calculation

Most current pulsed neutron density algorithms use inelastic gamma rays [25, 24]. However, the net inelastic gamma ray may not always be acquired as an input for practical applications, which increases the error of the density measurement algorithm. To demonstrate the practicality of the capture gamma correction method, the formation densities are calculated separately using the corrected count ratios versus the original count ratios (Eq. (22)). Because the density accuracy is an important index for evaluating density measurement-related methods, the calculated formation densities are compared with the true densities to illustrate the differences before and after the application of the method. Most pulsed neutron density logging uses a duty cycle of 20%; therefore, this is selected as the modelling parameter. Fig. 16 shows the results of the density calculations for this case. The model shown in the figure contains seven rocks: limestone, sandstone, dolomite, anhydrite, illite, kaolinite, and montmorillonite. The pore fluids are fresh water, methane, and oil. The formation bulk density ranged from 1.67 to 2.87 g/cm3.

Fig. 16
(Color online) Formation density calculation results at 20% duty cycle. Track1: Comparison of the true density with the formation density calculated using inelastic gamma count ratios through capture-correction method. Track2: Comparison of the true density with the formation density calculated using burst-on count ratios. Track3: Absolute error = |true density – calculated density 1|. Track4: Absolute error = |true density – calculated density 2|.
pic

In Fig. 16, the errors of the formation density calculated after the capture correction are all less than 0.025 g/cm3, whereas only 64% of the formation density results calculated using uncorrected gamma have an error of less than 0.025 g/cm3. In addition to absolute errors, the RMSE (Eq. (26)) is used as an indicator to evaluate the density accuracy where num is the number of samples, RMSE=1numi=1n(yiy^i)2, (26) yi denotes calculated density, and y^i  denotes true density.

The RMSE of the formation density calculated after the capture correction is 0.013 g/cm3, while the RMSE of the formation density calculated using burst-on count ratios is 0.025 g/cm3. The absolute error of the results obtained using the method proposed in this study is less than 0.025 g/cm3, and its RMSE is smaller than the RMSE without the capture correction, indicating that the method can effectively improve the accuracy of source-less density logging.

4

Conclusion

Conventional density measurement methods that use radioactive isotopes carry significant risks, including environmental contamination. Consequently, there is a growing interest in using manually controlled pulsed-neutron sources as an alternative method for source-less density measurements. However, the accuracy of source-less density measurements can be compromised by the presence of capture gamma rays during the neutron burst-on period. To overcome this challenge, this study introduced an adaptive capture gamma correction method for complex and diverse formation environments with varying pulse duty cycles. The results are as follows:

(1) The differential of the time spectra was calculated to identify and match the different neutron pulsed duty cycles. The capture time spectrum was calculated by introducing GPR, and the net inelastic gamma was obtained.

(2) For validation, a theoretical density tool was employed at different duty cycles in simulated environments with different porosities, pore fluids, and lithologies (288 model sets). Compared to the true inelastic gamma collected using the physical process, a consistent net inelastic gamma was obtained in 97.6% of the models under different environments and pulse duty cycles using the proposed method, which demonstrates the adaptability of the method.

(3) The errors of the formation density calculated after the capture correction were all less than 0.025 g/cm3, whereas only 64% of the formation density results calculated using uncorrected gamma had an error of less than 0.025 g/cm3.

These results show that the proposed method can effectively improve the accuracy of source-less density logging when the duty cycle and formation environment change. In future work, the feasibility of the proposed method will be explored further using a designed source-less density tool and field tests.

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