Introduction
Neutrons have been used in many scientific fields since they were discovered by Chadwick in 1932, making neutron detection technology vital for a variety of applications. Examples include nuclear reactors [1,2], meteorology [3], national security [4,5], astronautics [6], biology [7], and radiopharmaceuticals [8]. Detecting neutrons and monitoring neutron flux are vital tasks in the aforementioned fields. However, several radiation detectors that are sensitive to neutrons are additionally sensitive to high-energy photons (gamma rays). These photons inevitably accompany neutrons because of their interaction with the surrounding environment. This concomitant phenomenon causes difficulty in detecting neutrons because detectors retrieve the radiation pulse signals of neutrons and gamma rays simultaneously, making it particularly difficult to count only neutrons per unit of time. To overcome this obstacle, researchers have attempted to discriminate neutrons and gamma rays through their different interaction characteristics with the sensitive volume of a radiation detector, which can be presented by the differences in the pulse shapes of these two particles [9]. Based on this discrimination principle, the pulse shape discrimination (PSD) technique has been developed [10,11], which has been commonly used in numerous scientific fields to satisfy the neutron detection requirements [12,13]. One of the most important components of the PSD technique is its discrimination algorithm. This algorithm is responsible for the information extraction process of each radiation pulse signal, generating a discrimination factor for each signal, which is used to separate the neutron and gamma-ray pulse signals (n-
Many discrimination methods have emerged during the past decades, such as the most commonly used charge comparison (CC) method [14], fast discrimination-capable zero-crossing (ZC) method [15,16], frequency-domain-based frequency gradient (FGA) method [17] and fractal spectrum method [18]. The CC method is among the most frequently used PSD methods. It exhibited good discrimination performance under various conditions with low time consumption. The most significant advantage of the ZC method is its low computational complexity, making it a better option for real-time discrimination tasks. However, the discrimination performance of the ZC method is usually unsatisfactory because its information extraction process is too simple to fully determine the differences between pulse signals. Frequency-domain-based methods play an essential role in high-noise scenarios. Nevertheless, their computational burden is usually high and they require a long signal processing time. In 2021, Liu et al. proposed a novel discrimination method with outstanding discrimination performance [19], introducing a pulse-coupled neural network (PCNN) into the neutron and gamma-ray pulse-shape discrimination field for the first time. The PCNN displayed breakthrough discrimination performance and significantly outperformed conventional discrimination algorithms, such as the CC and ZC methods. The outstanding discrimination effect of the PCNN was attributed to its dynamic information extraction ability. As a biological neurology research-based neural network, the PCNN was initially conceived to imitate the working style of the biological neuron cortex to obtain the capability of processing dynamic information from pictures or videos [20]. In the biological visual system, when external light sources stimulate photoreceptor cells in the retina, these cells generate electrical signals (spikes) and relay these spikes to the adjacent optic nerves. These electrical signals stimulate neurons in the cortex, causing further spike generation and transmission between cell assemblies [21,22]. Biological neurology research has corroborated that this spike behavior between cell assemblies can recognize the information contained by the original stimuli received by the photoreceptor cells and makes the brain understand features, details, and other information in images or videos [23]. Inherited from this working style, the PCNN can similarly extract the dynamic information of images. As the PCNN was proposed by Johnson et al. in 1994, it has been used in numerous image-processing fields [24]. Examples include object recognition [25,26], image shadow removal [27], and image feature extraction [28].
Although Liu et al. demonstrated the discrimination effect of this PCNN-based method [29], its high computational complexity limited its rapid discrimination applications. This computational burden is a result of two factors: the high number of iterations of the PCNN and the integration process of the ignition map. Consequently, the computational burden of the PCNN-based discrimination method should be reduced, which requires a novel discrimination technique with a high information extraction ability and low computational complexity. In this study, a ladder gradient (LG) method was proposed. It replaces the integration process of the PCNN-based method with ladder gradient calculations. Moreover, a quasi-continuous spiking cortical model (QC-SCM) was proposed to generate ignition maps required for the ladder gradient calculation process. The QC-SCM can achieve a better-detailed information extraction performance and noise processing ability than the PCNN, with fewer number of iterations and manual parameters. Experiments were conducted to compare the discrimination results of the LG method with those of the other five conventional discrimination methods to evaluate the proposed method's efficiency and robustness.
Furthermore, the filtering process is a vital step in most PSD algorithms, that is, reducing the noise level of n-
The layout of this study is arranged as follows. The LG discrimination method principle is elaborated in Section 2. The filtering methods used are described in Section 3. Section 4 presents the evaluation criteria used to quantify the performance of the different filtering methods. The detailed structure of the experiments and experimental results are presented in Section 5. Finally, in Section 6, the conclusions of this study are presented.
Fundamentals of the ladder gradient method
Figure 1 shows a flow chart of the ladder gradient (LG)-based neutron and gamma-ray discrimination process. The radiation pulse signals (n-
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LG uses QC-SCM to generate the ignition maps of n-
Figure 2 shows a comparison of the pulse signals and ignition maps. The difference between the neutron and gamma-ray signals appeared in the falling edge (approximately 90 ns) and delayed fluorescence parts (approximately 180 ns), as shown in Fig. 2a. This difference was successfully captured and amplified by the PCNN, as shown in Fig. 2b, with generally higher ignition times in these two parts. However, the ladder shape ignition maps were unstable, with many fluctuations ranging from 100 to 200 ns. This fluctuation is caused by noise introduced by the radiation detection system. Although an integration process for the falling edge and delayed fluorescence parts can compensate for the noise-induced fluctuation, the computational complexity increment is an inevitable cost.
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In contrast, the QC-SCM ignition maps, as shown in Fig. 2c, did not show fluctuations in the ladder shapes. This stabilized ladder shape is formed because of the better noise-processing ability of the QC-SCM than that of the PCNN. A more computationally convenient discrimination factor than the integration, the ladder gradient, can be used because of the smooth ladder shape. Moreover, the QC-SCM can achieve a similar difference amplification performance as that of the PCNN with fewer iterations because of its better-detailed information extraction ability. The number of QC-SCM manual parameters is much lower than that of the PCNN. Similar to the PCNN, the QC-SCM requires no training process before discrimination.
Filtering methods
A one-dimensional signal can be considered a useful signal superposed by white Gaussian noise:
In practical applications, sampled signals are discrete-time signals with equal time steps. Consequently,
The noise-removal process extracts the useful signal
In this study, a total of 11 filtering methods and 20 filtering conditions were investigated to determine the optimal filters for the PCNN and LG methods. The details of these filtering methods are presented in Section S1 of Supplemental Information. These methods incorporate the Butterworth filter [32,33], Chebyshev filter [34,35], elliptic filter [36], median filter [37], moving average filter [38,39], Fourier filter [40], wavelet filter [41-44], Wiener filter [45,46], least mean square adaptive filter [47], morphological filter [48,49], and windowed-sinc filter [50,51].
Evaluation criteria
Figure of merit
The figure of merit (FoM) is a standard measurement used to evaluate the discrimination effect of neutrons and gamma rays [52]. The calculation of FoM first draws a histogram of discrimination results, which contains two groups corresponding to the gamma ray and neuron counts. Then, a Gaussian fitting function is used to fit these two groups, forming a fitting curve that can be further used to calculate the distance between these two peaks,
De-noised signal similarity measurements
There are several objective measurements of the denoising performance in image noise removal applications [53]. They can also be calculated in the one-dimensional condition to evaluate the de-noising performance of the radiation signals.
The peak signal-to-noise ratio (PSNR) measures the similarity between the denoised signal
The root mean square error (RMSE) can be calculated as,
The DIV can be used to measure the de-noising performance, which is defined as
Shannon entropy (SE) is a concept in information theory that can represent the average information contained in a signal [54,55]. It can be estimated as,
By calculating the SE of
Time consumption
The time consumption of the LG method and several other discrimination methods to process 9414 radiation pulse signals was measured. Furthermore, the time consumed by each filter to process all the signals was measured. Time consumption represents the computational complexity of the discrimination and filtering methods, indicating their implementation viability.
Discrimination accuracy
Determine whether the discrimination accuracy is influenced when n-
Smaller values of error and error ratio indicate better results.
Experimental procedures
Experiment equipment and parameter settings
This study used a 241Am-Be isotope neutron source with 4.5 MeV average energy to produce the radiation-superposed field. The n-
Five methods were compared with the LG method: falling edge percentage slope (FEPS) [57,58], zero crossing (ZC) [15,16], charge comparison (CC) [59], frequency gradient analysis (FGA) [17], and pulse-coupled neural network (PCNN) [19]. The parameters of these discrimination methods are presented in Sect. S2.1 of Supplemental Information.
The parameters of the filtering methods used in this study were optimized to achieve the near-best performance of each filter, and are presented in Sects. 2.2 and 2.3 of Supplemental Information.
Discrimination results and comparison
Figure 3 shows the discrimination performance. Discrimination is poorly performed by FEPS, as shown in Fig. 3a. Numerous pulse signals are located between the neutron and gamma-ray groups. The gradient of the two points at the peak of the signal and the end of the falling edge is used by the FEPS as the discrimination factor, similar to process of the LG method. However, without an information extraction process, noise significantly influences the discrimination performance of the FEPS. Additionally, the information inside the delayed fluorescence parts was not considered by FEPS. Consequently, it exhibits an unsatisfactory discrimination effect. Ignoring the delayed fluorescence parts influences the performance of the ZC method, as shown in Fig. 3b. Although the differentiation and integration processes help the ZC reduce noise interference, the incomplete pulse shape difference still causes a considerable negative impact, with a better Gaussian distribution of n-
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The discrimination performances of CC, FGA, and PCNN are better than those of the two aforementioned methods, as shown in Figs. 3c, 3d, and 3e. In the results of these three methods, the n-
The results of the objective evaluation are presented in Table 1. The results of the FoM values are consistent with the intuitive presentation of three-dimensional histograms. FEPS and ZC have the worst performance, with FoM values of approximately 1. The CC and FGA performances were at the same level. LG exhibits the second-best performance with a 1.54 FoM, which is slightly lower than the 1.75 FoM of the PCNN. The time consumption of each method was defined as the total CPU processing time for the 9414 pulse signals (the time consumption of the filtering process was excluded). The LG reduced the time consumption by approximately 37% compared with that of the PCNN, approaching the level of other conventional discrimination methods. These experimental results demonstrate the efficiency and robustness of the proposed LG method, which can achieve a better performance than conventional methods without preprocessing by filters and consumes less time than PCNN. The low computational complexity of LG makes it possible to implement integrated radiation detection systems, thereby realizing real-time discrimination.
Criteria/method | FEPS | ZC | CC | FGA | PCNN | LG |
---|---|---|---|---|---|---|
FoM (a.u.) | 0.97 | 1.09 | 1.38 | 1.47 | 1.75 | 1.54 |
Time consumption (s) | 1.28 | 1.36 | 1.30 | 1.31 | 2.78 | 1.76 |
Filtering results and analysis
We conducted experiments to validate the performance of the PCNN and LG coupled with each filter mentioned in Sect. 3. We evaluated their performance from four aspects: (A) discrimination performance (which is crucial in neutron and gamma-ray discrimination applications), (B) de-noised signal similarity (which measures the distortion), (C) time (referring to the total CPU processing time of each filter for all 9414 pulse signals), and (D) discrimination accuracy (which uses the most widely used discrimination and filtering method, that is, the CC method with a Fourier filter, as the reference, comparing its discrimination results with the results of other filters). There is no ground truth for the discrimination results because the n-
The distortion of a signal's peak and falling edge caused by different filters is shown in Fig. 4. As shown in Fig. 4a and 4b, the elliptic filter displayed a maximum change in the amplitude of the peaks, and the Butterworth filter smoothed the falling edge the best. As shown in Fig. 4c and 4d, the median filter significantly changed the shape of the signal's peak, and the moving average filter had the best performance in smoothing the falling edge. As shown in Fig. 4e and. 4f, the distortion of the peak in all three methods remains at the same level, whereas the wavelet filter outperforms the others in smoothing the falling edge. As shown in Fig. 4g and 4h, although the falling edges show the same characteristics after processing three different LMS filter conditions, the peak distortion of the model-reference condition is more extensive than that of the others. As shown in Fig. 4i and 4j, the morphological filters completely changed the characteristics of the pulse shapes with different peak shapes and locations. Finally, as shown in Fig. 4k and 4l, the model-reference Wiener filter significantly distorted the peak shape and performed poorly during the falling-edge smoothing process. The distortion of signals is acceptable in neutron and gamma-ray discrimination applications if the pulse shape difference between the neutrons and gamma rays is successfully preserved or amplified after the filtering process.
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The objective evaluation results for the three best filters of the PCNN and LG are presented in Tables 2 and 3, respectively. The detailed experimental results for all filters coupled with the PCNN and LG are presented in Sect. S3 of Supplemental Information.
Filtering methods | Evaluation criteria | |||||
---|---|---|---|---|---|---|
Wavelet | FoM | MSE | PSNR | RMSE | DIV | ED |
2.5915 | 7.83×10-5 | 41.4729 | 0.0086 | 0.0232 | 0.0233 | |
Distort | N-count | G-count | Error | Error ratio | Time (s) | |
0.0187 | 2050 | 7364 | 13 | 0.0014 | 5.7782 | |
Elliptic | FoM | MSE | PSNR | RMSE | DIV | ED |
2.1942 | 0.0053 | 22.7510 | 0.0728 | 0.1717 | 0.1567 | |
Distort | N-count | G-count | Error | Error ratio | Time (s) | |
0.1848 | 2065 | 7349 | 28 | 0.0030 | 1.2646 | |
Median | FoM | MSE | PSNR | RMSE | DIV | ED |
2.1811 | 0.0007 | 31.7574 | 0.0264 | 0.1937 | 0.0624 | |
Distort | N-count | G-count | Error | Error ratio | Time (s) | |
0.2231 | 2088 | 7326 | 51 | 0.0054 | 0.2351 |
Filtering Methods | Evaluation Criteria | |||||
---|---|---|---|---|---|---|
Elliptic | FoM | MSE | PSNR | RMSE | DIV | ED |
2.1956 | 0.0143 | 18.447 | 0.1196 | 0.1200 | 0.1400 | |
Distort | N-count | G-count | Error | Error ratio | Time (s) | |
0.1201 | 1929 | 7485 | 126 | 0.0134 | 1.2646 | |
Moving Average | FoM | MSE | PSNR | RMSE | DIV | ED |
1.6637 | 0.0063 | 22.0353 | 0.0791 | 0.0959 | 0.0759 | |
Distort | N-count | G-count | Error | Error ratio | Time (s) | |
0.0926 | 1899 | 7515 | 150 | 0.0159 | 0.1897 | |
Wavelet | FoM | MSE | PSNR | RMSE | DIV | ED |
1.6587 | 7.83×10-5 | 41.4729 | 0.0086 | 0.0232 | 0.0233 | |
Distort | N-count | G-count | Error | Error ratio | Time (s) | |
0.0187 | 2000 | 7414 | 107 | 0.0114 | 5.7782 |
Pertaining to the PCNN, the experimental results showed that the LMS and Wiener filters performed poorly regardless of the reference signal used. The time consumption of their model-reference conditions is inferior because it takes a considerable amount of time to fit 9414 pulse signals using the three-decay-exponential function. Although the filtered signals of these two filters are the most similar to the original signals, with the best denoised signal similarity measurements, they failed to preserve the difference between neutrons and gamma rays and hence showed an unsatisfactory discrimination effect. The moving average filter had the shortest discrimination time while presenting an acceptable discrimination performance. The Fourier filter is the most balanced filter, which showed good discrimination results and the best denoised signal similarity.
Furthermore, the three filters with the best discrimination performance, that are, wavelet, elliptic, and median are shown in Table 2. The wavelet filter presented the FoM, which significantly outperformed the other filters. It also has small signal distortion and a low discrimination error. The only drawback is that its time consumption is not the highest among all the filtering methods. The elliptic filter has the second-best discrimination performance, low discrimination error, and a short filtering time requirement. The main disadvantage of this filter is that its parameters need to be reset for different neutron sources or scintillators, which makes its application inconvenient. The median filter showed the third-best discrimination performance and the second-best filtering time. The major drawback of this filter is that signal distortion is relatively high.
LG cannot discriminate the n-
Table 3 lists the filters with the best discrimination performance (elliptic, moving average, and wavelet). The elliptic filter exhibited the best discrimination performance, with the highest FoM, minimal signal distortion, and fast discrimination time. The primary disadvantage is the manual parameters. The moving average filter achieved the lowest time consumption and the second-best FoM. Finally, the wavelet filter presented the best discrimination performance and denoised signal similarity. The primary drawback of this method is its high computational complexity.
Conclusion
This study proposes an LG method for neutron and gamma ray pulse shape discrimination. This method uses a computationally convenient process, that is, the ladder gradient calculation process, to obtain the discrimination factor. Furthermore, QC-SCM was proposed to generate the ignition maps required by the ladder gradient calculation. Experiments were conducted to compare the proposed method with five other discrimination methods: falling-edge percentage slope, zero crossing, charge comparison, frequency gradient analysis, and pulse-coupled neural network. The experimental results demonstrate the robustness and efficacy of the LG method, with the second-best FoM and low computational complexity.
Moreover, the filter adaptability of the PCNN and LG methods was investigated. Their performance was evaluated using both subjective figures and objective evaluation criteria. The evaluation criteria had the following four aspects:
· discrimination performance (FoM)
· De-noised signal similarity (signal-to-noise ratio, mean square error, root mean square error, DIV, and entropy difference)
· time (total time consumption for each filter to process all 9414 signals)
· discrimination accuracy (neutron pulse signal count, gamma-ray pulse signal count, error, and error ratio)
The advantages and disadvantages of various filters and the possible reasons for their adaptability were analyzed. The experimental results revealed that the wavelet, elliptic, and median filters were the most adaptive of the PCNN; and the elliptic, moving average, and wavelet filters were the most suitable for the LG. In future research, the LG method will be further optimized and implemented on integrated radiation detection systems, and the LG parameters will be studied to provide an automatic parameter LG method.
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