Gaseous products of aqueous <italic style="font-style: italic">N</italic>, <italic style="font-style: italic">N</italic>-dimethyl hydroxylamine degraded by radiation

Jinhua WANG; Chun LI; Minghong WU; Gang XU; Borong BAO; Weifang ZHENG; Hui HE; Shengdong ZHANG

doi:10.13538/j.1001-8042/nst.21.233-236

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Gaseous products of aqueous N, N-dimethyl hydroxylamine degraded by radiation

RADIOCHEMISTRY, RADIOPHARMACEUTICALS AND NUCLEAR MEDICINE | Updated：2021-01-29

- Gaseous products of aqueous N, N-dimethyl hydroxylamine degraded by radiation
- Nuclear Science and Techniques Vol. 21, Issue 4, (2010)
- Affiliations：
  
  1.Shanghai Applied Radiation Institute, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China
  2.Department of Radiochemistry, China Institute of Atomic Energy, Beijing 102413, China
- Author bio：
  
  Corresponding author. E-mail address:jinhuawang@staff.shu.edu.cn
  
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- DOI：10.13538/j.1001-8042/nst.21.233-236 CLC：
- Published：20 August 2010，
  
  Received：05 October 2009，
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Cite this article
Jinhua WANG, Chun LI, Minghong WU, et al. Gaseous products of aqueous N, N-dimethyl hydroxylamine degraded by radiation. [J]. Nuclear Science and Techniques 21(4):233-236(2010)
DOI：

Jinhua WANG, Chun LI, Minghong WU, et al. Gaseous products of aqueous N, N-dimethyl hydroxylamine degraded by radiation. [J]. Nuclear Science and Techniques 21(4):233-236(2010) DOI： 10.13538/j.1001-8042/nst.21.233-236.

Gaseous products of aqueous N , N -dimethyl hydroxylamine degraded by radiation 1 corresp first-author Corresponding author. E-mail address:jinhuawang@staff.shu.edu.cn Corresponding author. E-mail address:jinhuawang@staff.shu.edu.cn jinhuawang@staff.shu.edu.cn 1 1 1 1 2 2 2 Shanghai Applied Radiation Institute, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China Shanghai Applied Radiation Institute, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China Department of Radiochemistry, China Institute of Atomic Energy, Beijing 102413, China Department of Radiochemistry, China Institute of Atomic Energy, Beijing 102413, China In this work, the 0.1–0.5 mol·L –1 N, N-dimethylhydroxylamine (DMHA) were irradiated to 5–25 kGy, and gaseous products of mainly hydrogen, methane, ethane and n-butane were measured by gas chromatography. The results show that the volume fraction of hydrogen and methane increases with the concentration of DMHA and dose, and the latter does not change markedly at high doses. N N-dimethyl hydroxylamine Radiation degradation Gaseous product Spent fuel reprocess References Biddle P , Miles J H . J Inorg Nucl Chem , 1968 , 30 : 1291 - 1297 . J Inorg Nucl Chem Sze Y K , Gosselin J A . Nucl Technol , 1983 , 63 : 431 - 441 . Nucl Technol Sze Y K , Clegg L J , Gerwimg A F , et al . Nucl Technol , 1982 , 56 : 527 - 534 . Nucl Technol Biddle P , Mckay H A C , Miles J H . Solvent extraction chemistry of metals , Proc. Int. Conf. on solvent extraction of metals. Harwell , Macmillan, London . 1965 , 133 - 154 . Solvent extraction chemistry of metals Mckibben J M , Bercaw J E . 1971 , DP-1248 : 1 - 22 . Schlea C S , Caverly M R , Henry H E , et al . 1963 , DP-808 : 1 - 20 . Ochsenfeld W , Petrich G . Sep Sci Tech , 1983 , 18 : 1685 - 1698 . Sep Sci Tech Koltunov V S , Baranov S M , Zharova T P . Radiokhimiya , 1993 , 35 : 79 - 84 . Radiokhimiya Koltunov V S , Liu Y . J Radioan Nucl Chem , 2000 , 245 : 357 - 361 . J Radioan Nucl Chem Koltunov V S . Problems and Outlook RECOD’ 98 : 425 - 431 . Problems and Outlook RECOD’ Koltunov V S , Baranov S M , Zharova T P . Radiokhimiy , 1993 , 35 : 49 - 53 . (in Russian) Radiokhimiy Zhang A Y , Hu H X , Zhang Z Y , et al . J Radioanal Nucl Chem , 1998 , 230 : 235 - 239 . J Radioanal Nucl Chem Zhang A Y , Hu J X , Zhang X Y , et al . J Radioan Nucl Chem , 2002 , 252 : 565 - 571 . J Radioan Nucl Chem Zhang A Y , Hu J X , Zhang X Y , et al . J Radioan Nucl Chem , 2002 , 253 : 107 - 113 . J Radioan Nucl Chem Zhang A Y , Hu J X , Zhang X Y , et al . Solvent Extr Ion Exch , 2001 , 19 : 965 - 979 . Solvent Extr Ion Exch Zhang A Y , Hu J X , Zhang X Y , et al . At Energy Sci Tech , 2001 , 35 : 83 - 90 . (in Chinese) At Energy Sci Tech Wang J H , Li C , Bao B R , et al . Radiat Phys Chem , 2009 , 78 : 145 - 147 . Radiat Phys Chem Wang J H , Wan Y , Wu M H , et al . Nucl Sci Technol , 2008 , 19 : 343 - 346 . Nucl Sci Technol Wang J H , Wang S X , Bao B R , et al . Nucl Sci Technol , 2008 , 19 : 79 - 82 . Nucl Sci Technol Wang J H , Bao B R , Wu M H , et al . J Radioan Nucl Chem , 2004 , 262 : 451 - 453 . J Radioan Nucl Chem Wang J H , Bao B R , Wu M H , et al . J Nucl Radiochem , 2006 , 28 : 249 - 252 . (in Chinese) J Nucl Radiochem Wang J H , Bao B R , Wu M H , et al . J Nucl Radiochem , 2004 , 26 : 103 - 107 . (in Chinese) J Nucl Radiochem Wang J H , Bao B R , Wu M H , et al . J Nucl Radiochem , 2003 , 25 : 244 - 247 . (in Chinese) J Nucl Radiochem Wang J H , Bao B R , Wu M H , et al . J Radioan Nucl Chem , 2007 , 273 : 371 - 373 . J Radioan Nucl Chem Wu J L , Qi S C . Radiation Chemistry , Beijing Atomic Energy Publisher , 1993 , 156 - 198 . (in Chinese) Radiation Chemistry Spinks J W T , Woods R J . An introduction to radiation chemistry , 2 nd Ed. New York , A Wiley-Interscience Publication, John Wiley & Sons , 1976 , 247 - 295 . An introduction to radiation chemistry Wang J H , Wu M H , Bao B R J , et al . Nucl Technol , 2004 , 27 : 1 - 304 . (in Chinese) Nucl Technol Cheng H Y , Xiang C L , Chen Y H . At Energy Sci Technol , 1964 , 7 : 767 - 773 . (in Chinese) At Energy Sci Technol 10.13538/j.1001-8042/nst.21.233-236 Supported by Natural Science Foundation of China (Contract No.20771074) and Shanghai Leading Academic Disciplines (Contract No.S 30109) . 2009-10-05 2010-08-20 2021-01-19 2010 Nuclear Science and Techniques 04 21

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