Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO<sub>2</sub> interface

Huan Zhang

doi:10.1007/s41365-023-01256-6

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Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface

NUCLEAR CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR MEDICINE | Updated：2023-08-16

- Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface
- Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface
- 核技术（英文版） 2023年34卷第7期文章编号：108
- Affiliations：
  
  1.Instrumentation and Service Center for Physical Sciences, Westlake University, Hangzhou 310024, China.
  2.Shanghai Synchrotron Radiation Faciality, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201204, China.
  3.Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China.
- Author bio：
  
  * xiel@sari.ac.cn;
  songfei@sinap.ac.cn
- Funds：
  
  National Natural Science Foundation of China(11874380;22002183);National Key Research and Development Program of China(2021YFA1600800)
- DOI：10.1007/s41365-023-01256-6
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Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface[J]. 核技术（英文版）, 2023, 34(7):108

Huan Zhang, Lei Xie, Zhao-Feng Liang, et al. Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface[J]. Nuclear Science and Techniques, 2023, 34(7):108
Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface[J]. 核技术（英文版）, 2023, 34(7):108 DOI： 10.1007/s41365-023-01256-6.

Huan Zhang, Lei Xie, Zhao-Feng Liang, et al. Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface[J]. Nuclear Science and Techniques, 2023, 34(7):108 DOI： 10.1007/s41365-023-01256-6.

摘要

Abstract

Bimetallic catalysts typically exploit unique synergetic effects between two metal species to achieve their catalytic effect. Understanding the mechanism of CO oxidation using hybrid heterogeneous catalysts is important for effective catalyst design and environmental protection. Herein, we report a Bi-Au/SiO,2, tandem bimetallic catalyst for the oxidation of CO over the Au/SiO,2, surface, which was monitored using near-ambient-pressure X-ray photoelectron spectroscopy. The Au-decorated SiO,2, catalyst exhibited scarce activity in the CO oxidation reaction; however, the introduction of Bi to the Au/SiO,2, system promoted the catalytic activity. The mechanism is thought to involve the dissociation O,2, molecules in the presence of Bi, which results in spillover of the O species to adjacent Au atoms, thereby forming Au,δ+,. Further CO adsorption, followed by thermal treatment, facilitated the oxidation of CO at the Au-Bi interface, resulting in a reversible reversion to the neutral Au valence state. Our work provides insight into the mechanism of CO oxidation on tandem surfaces and will facilitate the rational design of other Au-based catalysts.

关键词

Keywords

APXPSCO oxidationAu-Bi interfaceTandem catalysisIn-situ

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Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO2 interface

Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO2 interface

DOI：10.1007/s41365-023-01256-6

摘要

Abstract

关键词

Keywords

references

Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface

Tandem catalysis for enhanced CO oxidation over the Bi-Au-SiO₂ interface