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Constraining nuclear symmetry energy with the charge radii of mirror-pair nuclei

NUCLEAR PHYSICS AND INTERDISCIPLINARY RESEARCH

Constraining nuclear symmetry energy with the charge radii of mirror-pair nuclei

Rong An
Shuai Sun
Li-Gang Cao
Feng-Shou Zhang
Nuclear Science and TechniquesVol.34, No.8Article number 119Published in print Aug 2023Available online 21 Aug 2023
46505

The nuclear charge radius plays a vital role in determining the equation of state of isospin asymmetric nuclear matter. Based on the correlation between the differences in charge radii of mirror-partner nuclei and the slope parameter (L) of symmetry energy at the nuclear saturation density, an analysis of the calibrated slope parameter L was performed in finite nuclei. In this study, relativistic and non-relativistic energy density functionals were employed to constrain the nuclear symmetry energy through the available databases of the mirror-pair nuclei 36Ca-36S, 38Ca-38Ar, and 54Ni-54Fe. The deduced nuclear symmetry energy was located in the range 29.89–31.85 MeV, and L of the symmetry energy essentially covered the range 22.50–51.55 MeV at the saturation density. Moreover, the extracted Ls at the sensitivity density ρs=0.10 fm3 was located in the interval range 30.52–39.76 MeV.

Symmetry energyCharge radiiMirror nuclei
1

Introduction

Precise knowledge of nuclear symmetry energy (NSE), which is characterized as a component of the equation of state (EoS) of isospin asymmetric nuclear matter, can provide access to various physical phenomena relevant to a broad range of density profiles and energy scales [1, 2]. NSE plays an important role in understanding the nuclear structure. Moreover, the behavior of NSE may affect the properties of neutron stars [3-5] and help to comprehend the supernova explosion mechanism and stellar nucleosynthesis in astrophysical studies [6].

The density dependence of NSE, that is, Es(ρ), can be expanded around the saturation density ρ0 (0.16 fm-3) as follows: Es(ρ)Es(ρ0)+L3(ρρ0ρ0)+Ksym18(ρρ0ρ0)2+, (1) where L and Ksym are the slope and curvature of the symmetry energy at the nuclear saturation density ρ0, respectively. The symmetry energy is believed to be associated with the isovector sensitive indicators in the EoS of isospin asymmetric systems. Unfortunately, a direct connection between the experimental observables and the EoS is not possible. Consequently, the microscopic implications of NSE can be extracted indirectly from the ground and the collective excited state properties of atomic nuclei, reaction observables, and detected dense astrophysical events [7, 8].

Thus far, enormous efforts have been undertaken to determine the EoS over the spread of density profiles and energy scales [9]. The neutron skin thickness (NST) of a heavy nucleus provides an available constraint on the EoS of neutron-rich matter around ρ0 [10-17]. In the laboratory, the radius of 208Pb has been detected by measuring parity-violating asymmetry in polarized elastic electron scattering experiments, for example sequentially in the PREX-II [18]. The accuracy of NST has been further updated from the latest performance, namely, Rskin208=0.283±0.071 fm. The behavior of Es(ρ) is mostly governed by the slope of the symmetry energy, L. The correlation between Rskin208 and the slope parameter L leads to a value of L=106±37 MeV [19]. In addition, NSE can also be investigated using the isotope binding energy difference [20, 21] and double magic nuclei [22, 23].

Significant progress has been made in evaluating NSE from the collective excited state properties of finite nuclei, such as isobaric analog states [24], pygmy dipole resonance (PDR) [25], electric dipole polarizability [26], giant dipole resonance (GDR) [27], isovector giant quadrupole resonance (IVGQR) [28], and charge-exchange giant resonance [29-32]. The results for L extracted from PDR in 68Ni and 132Sn were constrained to be in the intervals 50.3–89.4 MeV and 29.0–82.0 MeV [25], respectively. The deduced slope parameter from the weighted average can cover the range L=64.8 ±15.7 MeV. As suggested in Ref. [28], the slope parameter of the symmetry energy can be reduced to 37 ±18 MeV by exploiting IVGQR energies.

Moreover, NSE offers a key requirement for our understanding of nuclear reactions under isospin diffusions and isotopic distributions [33-35]. Heavy-ion collisions (HICs) provide a sensitive probe to link the nuclear EoS which depends on isovector potentials. In transport models, NSE is derived by simulating isospin-sensitive observables [36-40]. Hence, many simulation codes are desirable to determine the NSE [41-46]. More details about the transport simulations can be found in a recent study [47]. Meanwhile, new observations of compact stellar objects have provided plentiful data that help discern the EoS across saturation densities [48, 49]. The range of L can be deduced from the observation of dense object events, such as the production of gravitational waves from the neutron star merger GW170817 [50], resulting in L=11–65 MeV.

The density dependence of symmetry energy is fairly uncertain, except for the bulk properties at the saturation density ρ0. This challenges us in reducing the intrinsic uncertainties of the model from multiple aspects of the isovector components. As demonstrated in Refs. [51, 52], the difference in the root-mean-square (rms) charge radii of mirror-pair nuclei (ΔRch) obtained using Skyrme functionals provides an alternative opportunity for calibrating the density dependence of NSE.

A related linear correlation between ΔRch and the slope parameter L has been established. In Ref. [53], the differences in the charge radii of the mirror-partner nuclei 36Ca-36S and 38Ca-38Ar were investigated with varied values of L. It is evident that the slope parameter lies in the range L=5–70 MeV. The latest precise determination evaluated the correlation between the difference in charge radii of the mirror-partner nuclei 54Ni-54Fe and the slope parameter, which implied a range of L=21–88 MeV [54]. The rms charge radii of the nuclei 54Ni and 54Fe were obtained using Skyrme energy density functionals (EDFs) and covariant density functional theories (CDFTs), respectively.

As demonstrated above, ΔRch of mirror-pair nuclei can be employed to extract information about L. The latest results of the charge radii of 54Ni can facilitate efficient exploration of the nuclear EoS. The experimental data for Rch and ΔRch of the corresponding mirror partners are listed in Table 1 [53-55]. The NSE characterized as an isovector indicator in effective interactions should be systematically evaluated based on the latest experiments. To further obtain a comprehensive conclusion about the correlations between L and ΔRch, ΔRch for the pairs of mass numbers A=36, 38, and 54 can be calculated using non-relativistic and relativistic (covariant) EDFs. Although the correlations between the incompressibility coefficients and isovector parameters are generally weaker than the correlations between the slope parameter L and symmetry energy [56], the uncertainty suffered from nuclear incompressibility is inevitable in the evaluated process. Therefore, the values of incompressibility coefficients characterized as isoscalar parameters are almost identical for the two types of EDFs.

Table 1
Rch and ΔRch database for the A=36, 38, and 54 mirror-pair nuclei. The parentheses beside the values of charge radii and the difference in charge radii are systematic uncertainties [53-55].
A   Rch (fm) ΔRch (fm)
36 Ca 3.4484(27)
  S 3.2982(12) 0.150(4)
38 Ca 3.4652(17)
  Ar 3.4022(15) 0.063(3)
54 Ni 3.7370(30)
  Fe 3.6880(17) 0.049(4)
Show more

The remainder of this paper is organized as follows: In Sec. 2, we briefly report the theoretical models. In Sec. 3, we present the results and discussion. Finally, a summary and an outlook are provided in Sec. 4.

2

Theoretical framework

In this study, we adopted two types of widely used nuclear density functionals to extract information about the nuclear matter EoS, namely, the sophisticated Skyrme and covariant EDFs. Both have achieved great success in describing the bulk properties of finite nuclei, such as binding energies and charge radii. For a detailed introduction to non-relativistic and relativistic EDFs, refer to Refs. [57-59]. In this paper, we briefly introduce the two nuclear density functionals. The effective interaction in sophisticated Skyrme-type EDFs, which is expressed as an effective zero-range force between nucleons with density-dependence and momentum-dependence terms, is as follows: [60, 61] V(r1,r2)=t0(1+x0Pσ)δ(r)+12t1(1+x1Pσ)[P'2δ(r)+δ(r)P2]+t2(1+x2Pσ)P'δ(r)P+16t3(1+x3Pσ)[ρ(R)]αδ(r)+iW0σ[P'×δ(r)P],(2) where r=r1r2 and R=(r1+r2)/2 are related to the positions of two nucleons, P=(12)/2i is the relative momentum operator and P is its complex conjugate acting on the left, σ=σ1+σ2, and Pσ=(1+σ1+σ2)/2 is the spin exchange operator. The quantities α, ti, and xi (i=0-3) represent the parameters of the Skyrme forces.

For covariant EDFs, the interacting Lagrangian density has the following form: [62, 63] L=ψ¯[iγμμMgσσγμ(gωωμ+gρτρμ+eAμ)]ψ+12μσμσ12mσ2σ213g2σ314g3σ414ΩμνΩμν+12mω2ωμωμ+14c3(ωμωμ)214RμνRμν+12mρ2ρμρμ+Λv(gρ2ρμρμ)(gω2ωμωμ)14FμνFμν. (3) Here, Ωμν=μωννωμ, Rμν=μρννρμgρ(ρμ×ρν), Fμν=μAννAμ, and M, mσ, mω, and mρ are the nucleon, σ, ω, and ρ meson masses, respectively. The quantities gσ, gω, gρ, g2, g3, c3, and e2/4π=1/137 are the coupling constants for the σ, ω, ρ mesons, and photons. The parameter set Λv represents the coupling strength between the ω and ρ mesons. Solving the Skyrme HF and Dirac equations on a spherical basis, one can obtain the eigenenergies and wave functions of the constituent nucleons, from which the bulk properties of the ground states can be obtained using this standard procedure [57-63].

In our applications, two families of parameter sets were adopted: the asy family for Skyrme EDFs [64] and the IUFSU family for covariant EDFs [65]. All of these effective forces were calibrated by fitting the parameters to specific observables of finite nuclei, such as binding energies and charge radii, and the isovector part of the EoS was generated in such a way that the symmetry energy remained at a fixed value (26 MeV) around a sensitivity baryon density of ρs0.10 fm-3; thus, the interactions were characterized by different values of the symmetry energy at saturation density. This procedure ensures that the quality of the fit cannot be contaminated and that all isoscalar observables remain unchanged, for example, the incompressibility coefficient almost equals 230 MeV. In Fig. 1, the density dependence behaviors of the symmetry energies are plotted using the relativistic and Skyrme EDFs. With increasing symmetry energy at the saturation density ρ00.16 fm3, the slope became larger for these two families of parameter sets. For the symmetry energy around the sensitivity density ρs=0.10 fm3, these values were almost unchanged. Further details can be found in Refs. [65, 66]. It is worth mentioning that both the symmetry energies and slope parameters can cover a wide range. To reduce the intrinsic uncertainties of the models, such parameterization sets should be expected to provide stringent constraints on observables that are highly sensitive to the density dependence of the symmetry energy. The corresponding values of the bulk properties of the nuclear matter are shown explicitly in Table 2.

Table 2
Models used for the calculation of Rch. The corresponding bulk properties of nuclear matter used in this study, such as symmetry energy Es (MeV), the slope parameter L (MeV), and the incompressibility K (MeV) at saturation density, are given.
Type Sets Es (MeV) L (MeV) K (MeV)
RMF IUFSU05 30.48 46.11 229.98
  IUFSU04 31.52 52.09 229.98
  IUFSU03 32.59 60.52 230.05
  IUFSU02 33.85 71.83 230.01
  IUFUS01 35.49 87.27 230.04
  IUFSU00 37.16 108.76 229.88
Skyrme asy30 30.00 22.87 230.20
  asy32 31.99 36.22 229.99
  asy34 33.99 56.14 229.84
  asy36 36.00 71.54 229.93
  asy38 38.00 87.62 230.20
  asy40 40.01 106.09 230.09
Show more
Fig. 1
(Color online) Symmetry energies characterized by relativistic EDFS (a) and Skyrme EDFs (b) plotted as a function of density.
pic
3

Results and Discussion

The results for ΔRch are plotted as functions of L in Fig. 2. The non-relativistic Skyrme approach and RMF theory were used to assess the correlation between ΔRch and L, which are shown by the open circles and crosses in Fig. 2, respectively. The horizontal light blue bands indicate the uncertainties of ΔRch, which correspond to 0.146–0.154 fm (36Ca-36S), 0.060–0.066 fm (38Ca-38Ar), and 0.045–0.053 fm (54Ni-54Fe). The linear fits in the correction for ΔRch are indicated by the dashed lines.

Fig. 2
(Color online) ΔRch of the mirror-partner nuclei 36Ca-36S (a), 38Ca-38Ar (b), and 54Ni-54Fe (c) as a function of the slope parameter L at the saturation density ρ0. The experimental result is shown as a horizontal light blue band. The crosses are results of relativistic EDFs, and the open circles are for the Skyrme EDF calculations. The dashed lines indicate theoretical linear fits.
pic

The results obtained using the Skyrme and covariant EDFs revealed an approximate linear correlation between ΔRch and L. Constraints on L were deduced by comparing the theoretical predictions with the experimental results in Fig. 2. Note that the results for A=54 provided the slope of symmetry energy L relevant to the range 17.99–62.43 MeV, whereas those for A=38 and A=36 were in the intervals 6.83–52.49 and 22.50–51.55 MeV, respectively. We can see that these values essentially cover the theoretical uncertainties in Refs. [53, 54].

The NST of 48Ca is regarded as a feasible isovector indicator to constrain the EoS of nuclear matter. The high-resolution E1 polarizability experiment performed at RCNP suggests that the NST of 48Ca is located in the interval 0.140.20 fm [67]. Meanwhile, the CREX collaboration has reported a new value through parity-violating electron scattering measurements, namely, 0.0710.171 fm [68]. The NST of 48Ca allows a direct comparison to microscopic calculations using various slope parameters, L. In Refs. [69, 70], the linear correlation analysis of ΔRch of mirror-partner nuclei and the corresponding NST has been clearly illustrated. Therefore, it is essential to evaluate the correlations between ΔRch of mirror-pair nuclei and the NST of 48Ca.

The correlations between ΔRch of the A=36, 38, and 54 mirror-partner nuclei and the NST of 48Ca (ΔRnp) are also shown in Fig. 3. The calculated ΔRch substantially covered the current uncertainties of ΔRnp (48Ca) for both types of EDFs. For the A=54 mirror-pair nuclei, the Skyrme model gave a comparable correlation with respect to the RMF model. A high linear correlation between ΔRch of A=54 and ΔRnp of 48Ca was found. These correlations were also obtained using non-relativistic and relativistic EDFs for the A=36 and 38 mirror partners, as shown in Figs. 3 (a) and (b). This means that information on symmetry energy can be extracted from the differences in the charge radii of mirror-pair nuclei.

Fig. 3
(Color online) “ Data-to-data" relation between ΔRch of the A=36, 38, and 54 mirror-partner nuclei and the neutron skin thickness ΔRnp of 48Ca. The labels and color coding are the same as those used in Fig. 2.
pic

To obtain further constraints on the EoS of asymmetric nuclear matter, the relationship between the symmetry energy at saturation density and ΔRch of mirror-pair nuclei can also be evaluated as well as the relationship between L and ΔRch. Therefore, the “ Data-to-data" relationships between the symmetry energies and the slope parameters are shown in Fig. 4 via various colored planes for the A=36 (Ca-S), 38 (Ca-Ar), and 54 (Ni-Fe) mirror-partner nuclei. The shadowed plane represents the result of the theoretical prediction. From this figure, it is noticeable that the deduced symmetry energy was located in the interval Es=29.8931.85 MeV, and the slope of the symmetry energy covered the range L=22.5051.55 MeV. It should be mentioned that the present value provides a tighter constraint on L than those in Refs. [53, 54]. Although the mirror-partner nuclei for the masses A=36, 38, and 54 were simultaneously considered in our evaluated procedure, the effects of deformation and model uncertainties were not incorporated in our calculations as in Refs. [53, 54]. In forthcoming investigations, we will carefully study the effect of deformation on the charge radius of finite nuclei and estimate the model uncertainties using a comprehensive set of modern density functionals, which may change the present results.

Fig. 4
(Color online) Symmetry energy Es and the slope of symmetry energy L are limited by ΔRch of the A=36 (yellow plane), 38 (light purple panel), and 54 (light blue plane) mirror-partner nuclei. The shadowed plane represents the result of the theoretical prediction in this study.
pic

To facilitate the quantitative comparison of the extracted results with the theoretical calculations, various available estimates of the slope parameter L of the symmetry energy are shown in Fig. 5. It is evident that our present result has a remarkable overlap with the results obtained by various methods or observables. Our calculations predominantly covered the result for L extracted from PDR in 132Sn (L=29.0-82.0 MeV) but deviated from that of 68Ni (L=50.3-89.4 MeV) [25]. Figure 5 shows the weighted average value in the interval of 64.8±15.7 MeV. In addition, the electric dipole polarizability of a heavy nucleus is highly sensitive to both the magnitude and slope parameter of symmetry energy, providing a value of L=47.3±7.8 MeV [26]. By exploiting this correlation together with the experimental values of the isoscalar and isovector giant quadrupole resonance (GQR) energies, the slope parameter of the symmetry energy was estimated as L=37±18 MeV [28]. Both theoretical results essentially covered the current uncertainty in this study.

Fig. 5
(Color online) Comparison between the values of L extracted in this study and those from existing literature. We partly compare the values extracted from various models: Carbone et al. [25], Chen et al. [71], Steiner et al. [75], Roca-Maza et al. [28], Zhang et al [26], Mondal et al. [13], Raithel et al. [50], Brown et al. [53], Malik et al. [76], Zhang et al. [74], Pineda et al. [54], Newton et al. [80], and Tagami, et al. [72].
pic

The NST Δrnp in heavy nuclei provides an alternative terrestrial probe to place restrictions on the nuclear EoS. In Ref. [71], an accuracy value of L=58±18 MeV was deduced by analyzing the neutron skin data on Sn isotopes and the observables originating from HICs. Our calibrated results covered the uncertainty of this value. The latest NST of 48Ca detected by the CREX group yielded the slope parameter L=050 MeV [72], which is in accordance with this study (L=22.50-51.55 MeV). Significantly, the NST of 208Pb detected by the PREX-II group yielded a larger value of L=76165 MeV. Reed et al. [19] reported a comparable interval of the slope parameter L=106±37 MeV. These values partially cover the interval range of L=54~97 MeV induced by HICs [73]. However, the evaluated range in this literature has no overlap with the slope parameter L obtained by PREX-II.

In Ref. [74], more information, such as heavy-ion collision data, the neutron skin of 208Pb, tidal deformability, and the maximum mass of neutron dense objects, was used to calibrate the values of symmetry energy. This led to a symmetry energy slope of L=59.57±10.06 MeV, and the quantitative uncertainty was further reduced with respect to Ref. [71]. Moreover, the slope parameter L can be constrained by various observed astrophysical messages, except in terrestrial nuclear experiments. The currently available neutron star mass and radius measurements provide an important constraint on the EoS of neutron matter through quantum Monte Carlo simulations, in which the slope parameter L is located in the range 4352 MeV [75]. The correlation of the tidal deformability of a neutron star with L was studied using the sk Λ267 model, which gave the range L=41.1±18.2 MeV [76]. Moreover, the range L=11–65 MeV was extracted from the observation of a gravitational-wave event of the neutron star merger GW170817 [50]. Our calibrated range (L=22.5051.55 MeV) overlaps significantly with these deduced values.

Recently, emerging Bayesian frameworks have been developed widely to study the bulk properties of finite nuclei, for example, predictions in the nuclear charge radii [78, 77] and nuclear EoSs [79]. The existing database of neutron skin and the bulk properties of nuclear matter are characterized by prior input quantities, which leads to credible values of L=4026+34 MeV and L=378+9 MeV [80], respectively. All the evaluated values are consistent with the range of L obtained in this study.

As mentioned in Refs. [81, 82], the density dependence of the symmetry energy at the subsaturation density is associated with nuclear mass differences and multifragmentation production. Thus, it is also interesting to give the constraint of the slope parameter Ls at the sensitivity density ρs=0.10 fm3 probed by the differences in the charge radii of mirror-partner nuclei (ΔRch). In Fig. 6, ΔRch of the mirror-partner nuclei 36Ca-36S (a), 38Ca-38Ar (b), and 54Ni-54Fe (c) as a function of the slope parameter Ls at the sensitivity density ρs=0.10 fm3 are plotted. The highly linear correlations between ΔRch and Ls are also presented. The extracted interval range of the slope parameter Ls at the sensitivity density ρs=0.10 fm3 was approximately 30.52–39.76 MeV. This restricted value is relatively narrow compared to the interval range at the saturation density ρ00.16 fm3.

Fig. 6
(Color online) Same as Fig. 2, but for the slope parameter Ls at the sensitivity density ρs=0.10 fm3.
pic
4

Summary and outlook

Microscopic methods based on families of non-relativistic and relativistic EDFs were employed to characterize a systematic variation of the isoscalar and isovector properties of corresponding nuclear matter EoSs. Our systematic analysis of the extraction of the slope parameter L from the differences in mirror-partner nuclei charge radii provided a new result. The slope parameter L covered the interval range 22.50–51.55 MeV at the saturation density. Moreover, the slope parameter Ls at the sensitivity density ρs=0.10 fm3 lay in the interval range 30.52–39.76 MeV. This led to us determining the density dependence of symmetry energy relatively accurately, which is a fundamental quantity for nuclear physics and for the implications in the study of neutron stars.

Linear fits were performed between the differences in the charge radii of mirror-partner nuclei and the slope parameter L. As suggested in Refs. [83-87], precise descriptions of the nuclear charge radii are influenced by various mechanisms. Meanwhile, the precise measurement of the charge density distributions usually affects the NST of finite nuclei on a quantitative level. In Ref. [88], it is demonstrated that the differences in the charge radii of mirror-pair nuclei are systematically influenced by the pairing correlations. For weakly bound nuclei, configuration mixing should be discreetly considered when tackling pairing correlations [89]. Hence, this study should be further reviewed.

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Footnote

Feng-Shou Zhang is an editorial board member for Nuclear Science and Techniques and was not involved in the editorial review, or the decision to publish this article. All authors declare that there are no competing interests.