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Experimental study on the gas-stripping chamber of an E//B neutral particle analyzer

ACCELERATOR, RAY TECHNOLOGY AND APPLICATIONS

Experimental study on the gas-stripping chamber of an E//B neutral particle analyzer

Long Ma
De-Hao Xie
Yan-Xi Wang
Shuo Wang
Ji-Feng Han
Wei-Ping Lin
Jian-Li Liu
Xing-Quan Liu
Yu-Guo Liu
Xiao-Bing Luo
Yuan Luo
Guo-Feng Qu
Yu-Fan Qu
Pei-Pei Ren
Roy Wada
Lin-Ge Zang
Jing-Jun Zhu
Nuclear Science and TechniquesVol.35, No.11Article number 195Published in print Nov 2024Available online 12 Oct 2024
14304

Stripping units take a key role in the neutral particle analyzer (NPA). A renovated gas-stripping unit was constructed for the newly designed E//B NPA. Using H2 as the working gas, we measured the gas inlet pressure (P0) and vacuum chamber pressure (P3). The pressure distribution inside the gas-stripping room was calculated with Ansys Fluent, using the measured P0 and P3 as boundary conditions. The stripping efficiency of the stripping unit was then simulated utilizing the Geant4 Monte Carlo code for the H and D particles. The pressure P0=40 Pa, which is one-sixth of what found in the previous design and corresponds to a thickness of 1.27×1017 atoms/cm2, was obtained as the optimum working pressure for the upgraded stripping unit. An 50 kV electron cyclotron resonance (ECR) ion source platform was designed and constructed for E//B NPA calibration, and its performance has been measured. Using the ECR ion source platform, we measured the efficiency of the stripping unit through an inverse experiment with proton beams. We compared the current ratios of measurements with and without H2 gas to Geant4 simulation results. We found adequate agreement between the overall trends of the experiment and the simulation. The significant deviation for incident energies below 20 keV may result from the scattering effects of low-energy protons, leading to reduced accuracy in single-scattering physics in Geant4 simulations. Applying the scattering corrections observed in the reverse experiments obtains more accurate stripping efficiencies for H and D atoms in the energy range of 20-200 keV, and the global efficiency with the maximum values of 95.0% for H atoms and 78.9% for D atoms at 200 keV.

NPAGas-strippingECR ion sourceStripping efficiencyGeant4
1

Introduction

A tokamak is a magnetic-confinement fusion device used in controllable fusion experiments. The interaction between the shear Alfvén wave and energetic particles plays a crucial role in the high-temperature plasma confinement and steady-state operation of tokamaks [1-11]. Several diagnostic devices have been developed to study fusion plasma and the energetic particles on tokamaks, such as microwave diagnostics [12-14], soft X-ray diagnostics [15-17], neutron diagnostics [18-25], the visible/infrared camera [26-29], and the neutral particle analyzer (NPA) [30-37]. NPA is of great importance in providing energy spectra, which are key information for the frontier physics of energetic particles [4-6, 9, 38-40]. The bulk ion temperature, isotopic ratio, and fast-ion distribution of the plasma were obtained by measuring the charge exchange of neutral particles escaping from the plasma.

Since the first NPA was developed in 1960 [30], several NPAs have been designed and constructed worldwide [31-37, 41-50]. For example, the compact NPA (CNPA) [34] developed for the Wendelstein 7-AS stellarator offers the advantage of simultaneous analysis for hydrogen (0.8-80 keV) and deuterium (0.8-40 keV) with a more compact structure (size: 169 mm×302 mm×326 mm, weight: 42.5 kg). The NPA system on the international thermonuclear experimental reactor (ITER) includes a high-energy NPA to measure the D and T atoms within the energy ranges of 0.11 MeV to 1.4 MeV and 0.16 MeV to 2.2 MeV, respectively, and a low-energy NPA for the thermal energy range from 10 keV to 200 keV for all hydrogen isotopes [32, 48].

Typically, NPA comprises three main components: stripping, analyzing, and detection units. A stripping unit reionizes neutral particles via charge exchange reactions with the stripping material. The reionized particle energy and/or mass were identified by the magnetic and/or electric fields and recorded by the detecting unit. Various types of ion detectors [51], including micro-channel plates [35, 52-55], channel electron multipliers [34, 37, 56], CsI [31, 32, 50, 57, 58] LYSO scintillators [49, 59, 60], and diamond-like detectors [61, 62], are employed for the detecting unit of an NPA. The stripping material can be a stripping foil or gas. When using a solid foil as the stripping material in the NPA for low-energy neutrals, an additional accelerating or focusing voltage is often required for secondary ions [31, 32, 34]. Carbon foil with a thickness of 100 Å is commonly used as the stripping foil. In contrast, a gas chamber requires a differential pumping system when using a stripping gas. Typically, an integrated target with a thickness of the order of 1016 atoms/cm2 for H2 gas is used in the joint European torus (JET) NPA [44] and 1015 atoms/cm2 for He gas in the E//B NPA on TFTR [35]. This low-pressure operation is necessary to sustain a high vacuum level in the tokamak, resulting in low stripping efficiency.

A new NPA with parallel electric and magnetic fields (E//B) for studying the frontier physics of energetic particles is currently under development [63, 64]. A gas-stripping room filled with H2 as the working gas was adopted as the stripping unit in the E//B NPA. In a previous work Ref. [64], we presented the pressure distributions inside the stripping room simulated by Ansys Fluent [65, 66] and MolFlow+ [67]. The stripping efficiencies of H and D atoms passing through the stripping unit were then calculated using Geant4 [68, 69] simulation code. This study presents an experimental investigation of pressure distributions inside an upgraded stripping room, optimizing the initial design from [64, 70], and the ion beam tests of the stripping unit on a newly constructed 50 kV electron cyclotron resonance (ECR) ion source platform at Sichuan university.

The remainder of this paper is organized as follows. An experimental investigation of the pressure distribution inside the stripping room is presented in Section 2. Section 3 covers the newly constructed 50 kV ECR ion source platform and its performance. The ion beam tests of the stripping unit are detailed in Section 4. A brief summary is provided in Section 5.

2

Pressure distribution and stripping efficiency of the stripping unit

Our previous study presented a prototype design of the gas-stripping chamber [64, 70], where a stripping room with a length of 54 mm and two differential pipes with inner diameters of 4 mm was designed. The pressure distribution inside the stripping room was calculated using Ansys Fluent [65] and Molflow+ [67], assuming a constant pumping speed for the outlet surface. The stripping unit, constructed from a prototype design, exhibited reduced molecular pump speed when the pressure exceeded a certain value, resulting in higher vacuum chamber pressure compared to Ansys Fluent and Molflow+ calculations. Therefore, the stripping room structure was modified to reduce pressure in the vacuum chamber. An upgraded stripping room with a length of 84 mm and a differential pipes’ inner diameter of 2 mm was constructed for the stripping unit. Fig. 1 shows a cross-sectional view of the upgraded gas-stripping chamber.

Fig. 1
Cross-sectional view of the upgraded gas-stripping chamber
pic

Figure 2 shows a photograph of the upgraded stripping unit. A Faraday cup (FC) located in the downstream vacuum chamber was constructed, along with a stripping unit, to measure the incident beam current. A needle valve and an electromagnetic valve controlled by a proportional-integral-derivative (PID) controller were connected to the gas inlet flange to stabilize the H2 gas flow. Two diaphragm vacuum gauges, Pfeiffer CMR362 and CMR365 were used to measure the pressures of the gas inlet (P0) and vacuum chamber (P3), respectively. The pressure distribution inside the stripping room was obtained by applying the two measured pressures as the boundary conditions in Ansys Fluent.

Fig. 2
(Color online) Photo of the upgraded stripping unit
pic

By utilizing the experimentally measured P3 value in the Ansys Fluent calculations, a more accurate prediction of the pressure distribution inside the stripping room was obtained. Figure 3 shows a typical two-dimensional (2D) pressure distribution of P0=40 Pa on the central plane (Z=0 mm) of the stripping room in (a) and the pressure distribution along the incident neutral particles’ path (Y=0 mm and Z=0 mm) in the stripping room for P0=40 Pa in (b). With a reduction in the differential pipes’ inner diameter in the upgraded stripping unit, a higher pressure inside the stripping room is expected for a given P0. As shown in Fig. 3 (b), a constant pressure of approximately 31 Pa is applied in the center of the stripping room, which is more than three times that of the previous design [64]. The linearly decreasing pressures inside the differential pipes were also obtained.

Fig. 3
(Color online) (a) 2D pressure distribution of P0=40 Pa in the central plane (Z=0 mm) of the stripping room. (b) Pressure distribution along the path of the incident neutral particles (Y=0 mm and Z=0 mm) in the stripping room for P0=40 Pa. The inlet pressure (P0), the pressures of the center of the stripping room (P1), the inner end of the differential pipes (P2), and the vacuum chamber (P3) are indicated in the figure
pic

The pressures of the center of the stripping room (P1) and the inner end of the differential pipes (P2) were extracted and are shown together with P3 as a function of the inlet pressure P0 in Fig. 4. A linearly increasing trend of P1 is observed as the inlet pressure P0 increases, whereas slightly nonlinear changes in P2 and P3 are observed. This may result from variations in the pumping speed for different P0 values, leading to nonlinear changes in P2 and P3.

Fig. 4
(Color online) P1 (solid squares), P2 (solid triangles), and P3 (solid circles) as a function of P0. The solid curve is the linear fit of P1. Dashed and dotted curves are the second-order polynomial fit of P2 and P3, respectively. P3 is multiplied by a factor of 100 for easier comparison
pic

Geant4 [68, 69] Monte Carlo code was applied to simulate the global stripping efficiency (R×f+1, where R represents the transmission rate of the stripping room and f+1 is the fraction of the +1 charge state at the exit hole of the stripping chamber) of an earlier version of the stripping unit, and an optimum P0 pressure of 240 Pa were obtained in our previous work [64, 70]. In the simulation, the charge exchange cross sections of the ORNL recommended dataset [71] were employed, including the electron capture and loss cross sections of H0, the electron capture cross sections of H+, and the loss cross sections of H-. Taking the charge exchange cross sections at a given energy allows for obtaining the stripping efficiency from a simple equation without scattering corrections, as shown in Eq. (1) in [64]. The R×f+1 values were obtained by modifying the structure and pressure distribution in the code to match the upgraded stripping unit. Figure 5 shows R×f+1 as a function of the gas inlet pressure P0 for H and D atoms with incident energies 20 keV, 100 keV, and 200 keV in (a), (b), and (c), respectively. As the length of the stripping room increased, the thickness of the stripping gas increased in the upgraded stripping unit. Thus, a lower P0 value was required to achieve the same global stripping efficiency in the upgraded stripping unit. One can see from Fig. 5, the global efficiency increases with the gas inlet pressure P0, and reaches a maximum value of approximately 40 Pa for the maximum designed energy (200 keV) in the upgraded stripping unit. The optimum working pressure for the upgraded stripping unit was determined to be P0 = 40 Pa, five times lower than in the previous design [64], corresponding to a thickness of 1.27×1017 atoms/cm2.

Fig. 5
Global efficiency R×f+1 as a function of the gas inlet pressure P0 for incident energies 20 keV (a), 100 keV (b), 200 keV (c). The solid and open circles represent H and D, respectively
pic
3

The 50 kV ECR ion source platform

A new 50 kV ECR ion source platform with a compact permanent-magnet ECR ion source and a 30 dipole magnet was designed and constructed at Sichuan University to calibrate the E//B NPA. In general, the ion source platform consists of an ECR ion source, a dipole magnet, an FC, and vacuum and water-cooling systems. Figure 6 shows a photograph of the 50 ECR ion source platform.

Fig. 6
(Color online) Photograph of the 50 kV ECR ion source platform
pic

As shown in Fig. 7, a more compact and concise 2.45 GHz single-charge-state ECR ion source, modified from [72], was developed for the new 50 kV ECR ion source platform. The outer diameter of the source body was 50 mm. The magnetic field was produced by a single NdFeB permanent-magnet ring. A plasma chamber of diameter 30 mm and length 30 mm was designed for the ion source. The suppressor and shield electrodes described in [72] were removed from the ion source. The diameters of the plasma and extraction apertures were reduced to 3 mm and 5 mm, respectively. The newly designed spherical antenna head, which increased the plasma density in the chamber by approximately 10%, was used for the ion source. The length of the ceramic insulator tube was extended to 120 mm to sustain the 50 kV extraction voltage. The high-voltage power supply exhibited a 0.1% voltage drift over time and temperature. The microwave power source, placed on a high-voltage platform, was coupled to the plasma chamber via a coaxial cable and antenna. An isolation transformer rated for up to 80 kV and 1 kVA supplied power to the microwave generator. A needle valve with a leakage rate of 10-9 Pa·L·s-1 controlled the inlet flow of the working gas. The energy spread that was caused by the plasma instabilities in the extracted beam was measured by a retarding field energy analyzer revealed a maximum spread of less than 5 eV.

Fig. 7
(Color online) Structure drawing of the ECR ion source
pic

A dipole magnet with a deflection angle of 30, deflection radius of 250 mm, gap of 40 mm, and width of 70 mm was installed to analyze 50 keV He+ particles from the ECR ion source. As shown in the schematic of the 50 kV ECR ion source platform in Fig. 8, the ECR ion source and the dipole magnet were connected to a vacuum chamber (A). The other vacuum chamber (B) was located downstream of the dipole magnet. Two identical molecular pumps with pumping speeds of 700 L/s (N2) were mounted on the two chambers to maintain fine vacuum conditions. A collimator of diameter 5 mm was installed between Chamber A and the dipole magnet to reduce the beam spot after the dipole magnet. Using this collimator, a typical beam spot with a diameter of less than 15 mm was obtained for proton beams with an incident energy of 20 keV at the terminal flange. An FC with an entrance diameter of 2 cm was mounted in Chamber B to measure the beam intensity. The platform was equipped with a temperature-controlled deionized water-cooling system for the ion source and the dipole magnet.

Fig. 8
Schematic diagram of the ECR ion source platform
pic

The performance of the 50 kV ECR ion source platform was measured using hydrogen gas with 99.999% purity as the working gas. The beam current was measured using the FC in vacuum chamber B. The FC suppressor electrode was biased toward -300 V to suppress the secondary electrons. Fig. 9 shows the typical beam current as a function of the magnetic current for extraction voltages of 5 keV, 10 keV, 20 keV, and 40 keV in (a), (b), (c), and (d), respectively. The three large peaks from right to left are H3+, H2+, and H+. The two small peaks on the low-magnetic-current side are the breakup H+ events from H3+ (left) and H2+ (right). A small peak is observed between the largest H+ and H2+ peaks at an extraction voltage of 20 keV, corresponding to the breakup of H2+ from H3+. Rather small yields of breakup H2+ were found at other extraction voltages. Notably, the gas inlet flow changed for the above four extraction voltages, leading to a difference in the charged-particle yield shown in Fig. 9. The charged-particle composition should be further optimized for actual applications.

Fig. 9
Typical beam current as a function of the magnetic current for the extraction voltage 5 keV (a), 10 keV (b), 20 keV, (c) and 40 keV (d)
pic

The charged-particle intensity dependence on the microwave power was measured at a constant gas inlet flow and an extraction voltage of 5 keV. The gas inlet flow was monitored using the pressure measured in Chamber B. A constant pressure of PB=3.44×104 Pa was maintained throughout the measurements. The breakup of charged particles was ignored in this analysis because of low production yields. Fig. 10 shows the total, H+, H2+, and H3+ currents as functions of the microwave power. The total current was calculated by summing currents H+, H2+, and H3+. Figure 10 shows that the total current increased dramatically when the microwave power rose from 53 W to 146 W, which is consistent with the results in [72]. As microwave power increased, the fractions of H+ and H2+ rose, while H3+ decreased at powers above 120 W. This may be due to the increase in the electron density with higher microwave power [73], which produces more H2+.

Fig. 10
Total, H+, H2+, and H3+ currents as a function of the microwave power
pic

The dependence of the charged-particle intensity on the gas inlet flow was measured at a fixed microwave power of 95 W and an extraction voltage of 5 keV. Figure 11 shows the total, H+, H2+, and H3+ currents as functions of PB. The total current rapidly increased, peaking at PB=5.27×10-4 Pa and then gradually decreased as PB increased further. The H+ intensity increased smoothly with PB, peaking at the same PB value as the total current. The H2+ intensity peaked at a lower pressure of PB=3.7×10-4Pa, while H3+ dominated at PB above 5e-4Pa.

Fig. 11
(Color online) Total current, H+, H2+, and H3+ beam intensities as functions of PB
pic

A H3+ beam intensity comparable to that of H2+ was observed for all microwave powers, as shown in Fig. 10. At higher gas inlet flow rates, the H3+ fraction exceeded (more than 90%), as shown in Fig. 11. High H3+ fractions are reported in pulse-type ECR ion sources [74] but not in DC-mode ECR ion sources. Studies show that higher working gas pressure and lower microwave power in ECR ion sources increase H3+ production [74, 75]. The extremely high H3+ ion fraction in our 50 kV ECR ion source platform may result from the small discharge chamber and extraction hole, leading to higher pressure. This is significant for intense H3+-beam applications.

4

The experimental test of the gas-stripping unit

Calibration of the gas-stripping unit is crucial for the NPA. Direct verification of simulated results in the laboratory is challenging owing to the difficulty in handling neutral particles for precise measurements. However, because the stripping cross sections from neutrals to ions and the captured cross sections from ions to neutrals are comparable at a given energy [64], verification can be performed using ion beams in a reverse scenario.

Reverse experiments were conducted using the 50 kV ECR ion source platform. Figure 12 shows the schematic of the gas-stripping unit experimental setup on this platform. Proton beams with energies of 5 keV, 10 keV, 20 keV, 30 keV, and 40 keV were delivered to the gas-stripping unit. After charge exchange processes in an H2-filled stripping room, the total current of the remaining charged particles was measured using the FC located in the downstream chamber. A digital current integrator (ORTEC 439) measured the current of the charged particles in the FC, with the output pulse recorded by a CAEN DT5724B digitizer. The beam current without H2 gas was measured before and after each experiment as a reference. Experiments were conducted at gas inlet pressures of P0=20 Pa, 30 Pa, and 40 Pa for each incident proton energy.

Fig. 12
(Color online) Schematic diagram of the experimental setup of the gas-stripping unit on the 50 kV ECR ion source platform
pic

In the experiment, each ORTEC 439 pulse corresponded to 10-10 C. An FC current was recorded for each measurement. Fig. 13 shows the FC current as a function of the recording time for 20 keV incident protons. The solid circles, solid down triangles, and open squares represent the vacuum conditions in the stripping room at the beginning, middle, and end of the 20 keV proton measurements, respectively. The solid squares, solid triangles, and open circles represent measurements with filled H2 gas pressures of P0=40 Pa, 30 Pa, and 20 Pa, respectively. The solid lines indicate linear fits. A slight decreasing trend of less than 0.5% over the recording period for the three vacuum measurements suggests the long-term stability of the ECR ion source. Measurements under vacuum conditions before and after those with H2 gas serve as a reliable reference for the beam intensity of those with H2 gas.

Fig. 13
(Color online) FC current as a function of the recording time for 20 keV incident protons. Solid circles, solid down triangles, and open squares correspond to the vacuum condition in the stripping room at the beginning, middle, and end of 20 keV proton measurements; solid squares, solid up triangles, and open circles represent measurements with filled H2 gas pressure of P0=40 Pa, 30 Pa, and 20 Pa, respectively. Solid lines represent linear fits
pic

The current ratios for measurements with and without (vacuum) H2 gas were obtained from the FC currents ratios. The linear fit from vacuum measurements was used to extrapolate the beam currents for each H2 gas measurement. Fig. 14 shows the current ratio as a function of the proton energy (Ep) for P0=20 Pa (solid triangles), 30 Pa (solid squares), and 40 Pa (solid circles); Geant4 simulations with proton beams are presented for comparison. The ratio rapidly increased as Ep increased at Ep>10 keV and showed a flat trend at Ep≤10 keV. This trend is consistent with the electron removal cross section (σ0,1) shown in [71]. This was confirmed by a Geant4 simulation, in which the same overall trend was obtained. One can observe from Fig. 14, noticeable deviations between the simulation and experiment for the proton energy Ep≤20 keV. Geant4 simulations yielded nearly identical results for a given Ep across three different P0 values. This consistency may arise from accuracy limitations in single-scattering physics at energies below 20 keV, leading to significant deviations in the simulations. The E//B NPA was designed for an energy range of 20-200 keV, where scattering effects for low-energy particles are small for incident energies above 30 keV.

Fig. 14
(Color online) Current ratio of the measurements between with and without (vacuum) H2 gas as a function of the proton energy for P0=20 Pa (solid triangles), 30 Pa (solid squares), and 40 Pa (solid circles). The dotted, dashed, and solid curves are the Geant4 simulations for P0=20 Pa, 30 Pa, and 40 Pa, respectively
pic

The scattering effects from reverse experiments for low-energy (E≤30keV) protons were used to adjust the stripping efficiency from Geant4 simulations, as shown in Fig. 15. The global stripping efficiencies for H and D gradually increased with energy from 20 keV to 200 keV, reaching a maximum value of 95.0% for H atoms and 78.9% for D atoms at 200 keV. These results indicate that the upgraded stripping room has excellent stripping capability for H and D atoms within the energy range of 20 keV–200 keV at P0=40 Pa.

Fig. 15
Global efficiency R×f+1 as a function of the incident energy at P0=40 Pa. The solid and open circles represent H and D atoms, respectively
pic
5

Summary

An upgraded stripping unit of the newly designed E//B NPA was constructed. We measured the dependence of the vacuum chamber pressure (P3) on the gas inlet pressure (P0) and used these measurements as boundary conditions in Ansys Fluent to obtain the internal pressure distributions. The stripping unit efficiency was simulated using the Geant4 Monte Carlo code. Modifying the stripping room length from 54 mm to 84 mm and the inner radius of the differential pipes from 4 mm to 2 mm resulted in a central pressure (P1) over three times higher than that in the previous design. An optimal pressure of P0=40 Pa was achieved, which is reduced to one-sixth of the previous value and corresponds to a thickness of 1.27×1017 atoms/cm2.

A 50 kV ECR ion source platform was designed and constructed to calibrate the E//B NPA at Sichuan University. A more compact 2.45 GHz single-charge ECR ion source, capable of providing H+, H2+, and H3+ beams at energies below 50 keV was developed for this platform. Performance measurements with H2 as the working gas offer valuable insights for future applications.

The stripping efficiency of the stripping unit was investigated in the reverse scenario using the 50 kV ECR ion source platform. Instead of using neutral beams, proton beams with energies of 5 keV, 10 keV, 20 keV, 30 keV, and 40 keV were delivered to the stripping unit, which was filled with H2 gas at inlet pressures of P0=20 Pa, 30 Pa, and 40 Pa. The beam current was measured by an FC in the vacuum chamber located downstream of the stripping unit. The current ratios of the measurements with and without H2 gas were compared with those of Geant4 simulations. The experiment and simulation exhibited good overall agreement. The significant deviation at incident energies below 20 keV may stem from the differences between the scattering effect and the single-scattering physics of low-energy protons in Geant4 simulations. Considering this scattering effect, more accurate stripping efficiencies were obtained, with maximum global efficiencies of 95.0% for H atoms and 78.9% for D atoms at 200 keV.

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Footnote

The authors declare that they have no competing interests.