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Vol.30, No.7
NUCLEAR CHEMISTRY, RADIOCHEMISTRY, NUCLEAR MEDICINE
Research article 03 Jun 2019
Mohammed Sultan Al-Buriahi,Halil Arslan,Baris T. Tonguc
The mass energy-absorption coefficient (μen/ρ), effective atomic number (ZPEAeff), and electron density (NPEAeff) of some biomolecules with potential application in radiation dosimetry were calculated for their photon energy absorption (PEA) in the energy region of 1 keV to 20 MeV. It was noticed that the values of μen/ρ, ZPEAeff, and NPEAeff vary with the energy and composition of the biomolecules. The results for ZPEAeff were compared with effective atomic numbers (ZPIeff) owing to the photon interaction (PI). Significant differences were noted between ZPEAeff and ZPIeff in the energy region of 10 to 150 keV for all of the biomolecules involved. A maximum difference of 45.36% was observed at 50 keV for creatinine hydrochloride. Moreover, the studied attenuation parameters were found to be sharply affected at the K-absorption edge of relatively high-Z elements present in the biomolecules.
keywordElectron density;Effective atomic number;Photon energy absorption;Biomolecule;
Research article 04 Jun 2019
Mohammad W. Marashdeh,Hanan Saleh
The mass attenuation coefficients (μ/ρ) of a natural material, i.e. olive peat, were measured at photon energies of 0.059, 0.356, 0.662, 1.17, and 1.332 MeV and compared with those of concrete and Pb. The experimental samples were irradiated with 214Am, 133Ba, 137Cs, and 60Co point sources using a transmission arrangement. The olive peat samples were obtained from different areas in Jordan, namely Mafraq (sample M), Kerak (sample K), Ajloun (sample A), and Irbid (sample I), and photon energies were measured using a NaI(Tl) scintillation detector with an energy resolution of 7.6% at 662 keV. The differences in the µ/ρ of olive peat samples and the calculated µ/ρ of concrete were consistently within 0.7%. This finding indicates that olive peat can be used in radiation applications in the field of medical physics. Finally, the half-value layer (HVL) of the experimental samples was measured, and results were compared with those of concrete and Pb. Pb and concrete exhibited minimal X1/2 values due to their high density, and the HVL of olive peat revealed lower shielding effectiveness than that of concrete.
keywordgamma ray;Attenuation coefficient;Olive peat;Half-value layer;
Research article 12 Jun 2019
Hai-Bo Peng,Tie-Shan Wang,Xin Du,Tian-Tian Wang,Bing-Huang Duan,Xiao-Yang Zhang,Feng-Fei Liu,Chang-Lin Lan,Guang-Fu Wang,Liang Chen
Sodium borosilicate glasses are candidate materials for high-level radioactive waste (HLW) vitrification; therefore, understanding the irradiation effects in model borosilicate glass is crucial. Effects of electronic energy deposition and nuclear energy deposition induced by the impact of heavy ions on the hardness and Young's modulus of sodium borosilicate glass were investigated. The work concentrates on sodium borosilicate glasses, henceforth termed NBS1 (60.0% SiO2, 15.0% B2O3 and 25.0% Na2O in mol %). The NBS1 glasses were irradiated by P, Kr and Xe ions with 0.3 MeV, 4 MeV and 5 MeV respectively. The hardness and Young's modulus of ion-irradiated NBS1 glasses were measured by nanoindentation tests. The relationships between the evolution of the hardness, the change in the Young’s modulus of the NBS1 glasses, and the energy deposition were investigated. With the increase of the nuclear energy deposition, both the hardness and Young's modulus of NBS1 glasses dropped exponentially and then saturated. Regardless of the ion species, the nuclear energy depositions required for the saturation of hardness and Young's modulus were apparent at approximately 1.2×1020 keV/cm3 and 1.8×1020 keV/cm3, respectively. The dose dependency of the hardness and Young's modulus of NBS1 glasses was consistent with previous studies by Peuget et al. Moreover, the electronic energy loss is less than 4 keV/nm, and the electronic energy deposition is less than 3.0×1022 keV/cm3 in this work. Therefore, the evolution of hardness and Young's modulus could have been primarily induced by nuclear energy deposition.
keywordIrradiation;Hardness;Borosilicate glass;Young';s modulus;Nuclear energy deposition;
ACCELERATOR, RAY TECHNOLOGY AND APPLICATIONS
Research article 03 Jun 2019
Shu-Xin Zheng,Shyh-Yuan Lee,Hong-Jin Zeng,Hong-Juan Yao,Xue-Wu Wang,Hui Ning,Xiao-Jun Meng
The Xi’an Proton Accelerator Facility synchrotron lattice has a systematic fourth-order resonance. The systematic octupole component in dipole magnets is found to have no adverse effect on the dynamic aperture in multiparticle tracking. The frequency map shows particles locked onto the 2νx-2νz=0 resonance. However, we will show that the instantaneous betatron tunes can vary widely around the resonance line for particles locked onto the resonance.
keywordDynamic aperture;Octupole;Coupling resonance;XiPAF;
Research article 04 Jun 2019
Zhan-Shan Wang,Jia-Qi Chen,Qiu-Shi Huang,Run-Ze Qi,Yu-Fei Feng,Jiang-Tao Feng,Zhong Zhang,Wen-Bin Li
Gold films deposited by direct current magnetron sputtering are used for synchrotron radiation optics. In this study, the microstructure and surface roughness of gold films were investigated for the purpose of developing high reflectivity mirrors. The deposition process was first optimized. Films were fabricated at different sputtering powers (15, 40, 80, and 120 W) and characterized using grazing incidence X-ray reflectometry, X-ray diffraction, and atomic force microscopy. The results showed that all the films were highly textured, having a dominant Au (111) orientation, and the film deposited at 80 W had the lowest surface roughness. Subsequently, post-deposition annealing from 100 to 200 °C in a vacuum was performed on the films deposited at 80 W to investigate the effect of annealing on the microstructure and surface roughness of the films. The grain size, surface roughness, and their relationship were investigated as a function of annealing temperature. AFM and XRD results revealed that at annealing temperatures of 175 °C and below, microstructural change of the films was mainly manifested by the elimination of voids. At annealing temperatures higher than 175 °C, grain coalescence occurred in addition to the void elimination, causing the surface roughness to increase.
keywordMicrostructure;Roughness;Annealing;Gold films;Sputtering power;
Research article 06 Jun 2019
F. Akman,O. Agar,M.R. Kaçal,M.I. Sayyed
In this study, the gamma radiation shielding features of several environmentally-friendly materials were investigated. For this purpose, several attenuation parameters, such as the mass attenuation coefficient (μ/ρ), radiation protection efficiency (RPE), and effective atomic number (Zeff) were determined experimentally and compared with numerical data obtained using WinXCOM software. In the measurements, the emitted gamma photons were counted by a gamma spectrometer equipped with an HPGe detector using 22Na, 54Mn, 57Co, 60Co, 133Ba, and 137Cs radioactive point sources in the energy region of 81–1333 keV. The obtained results indicate that the μ/ρ and RPE values of the samples decrease with increasing photon energy. The experimental values are in good agreement with those obtained using WinXCOM software. The RPE and Zeff results show that, among the studied materials, the NaY0.77Yb0.20Er0.03F4 sample has the best gamma radiation shielding effectiveness.
keywordRadiation Shielding;WinXCom;Attenuation coefficient;Greener products;Radiation protection efficiency.;
Research article 12 Jun 2019
Li-Hua Wang,Mao-Lin Zhang,Li-Li Zhang,Hai-Sheng Yu
A shard of Chinese under-glaze copper-red porcelain from the Yuan dynasty (AD 1271-1368) made in the Jingdezhen kiln was measured by synchrotron radiation induced X-ray fluorescence (XRF) mapping and X-ray absorption near-edge spectroscopy (XANES) to investigate the influence of copper element distribution and speciation on the color of porcelain. In black-colored region, copper accumulates at the interface between the body and glaze layers with metallic copper particles as the main speciation. In contrast, Cu is irregularly distributed in the red-colored region with multi-valence speciation. The differences in Cu distribution and speciation in black- and red-colored regions indicate that they are the main factors influencing the different colors of copper-red under-glaze porcelain.
keywordCopper distribution and speciation;Chinese under-glaze copper-red porcelain;Synchrotron techniques;
Research article 15 Jun 2019
Zu-Jun Wang,Yuan-Yuan Xue,Min-Bo Liu,Rui Xu,Hao Ning,Wen Zhao,Bao-Ping He,Zhi-Bin Yao,Jiang-Kun Sheng,Wu-Ying Ma,Guan-Tao Dong
The objective of this work is to analyze the transient effects of 60Co gamma rays in the CMOS image sensor (CIS) using the Monte Carlo method, based on Geant4. The track, energy spectrum, and angle of produced electrons when gamma rays traversed an silicon or silicon dioxide cube were calculated. A simplified model of a 500×500 CIS array was established, and the transient effects of gamma rays in the CIS were simulated. The raw images were captured when the CIS was irradiated by gamma rays. The experimental results were compared with the simulation results. The characteristics of the typical events induced by transient effects were analyzed.
keywordGeant4;60Co gamma rays;Transient effects;CMOS image sensor (CIS);
SYNCHROTRON RADIATION TECHNOLOGY AND APPLICATIONS
Research article 04 Jun 2019
Qiang Gu,Jun-Jie Guo,Meng Zhang,Zhen Wang,Jian-Hao Tan
Shanghai high-repetition-rate XFEL and extreme light facility (SHINE), the first hard XFEL based on a superconducting accelerated structure in China, is now under development at the Shanghai Institute of Applied Physics, Chinese Academy of Sciences. In this paper, power losses caused by trapped longitudinal high-order modes (HOM), steady-state loss, and transient loss generated by untrapped HOMs in the 1.3-GHz SHINE cryomodule are investigated and calculated. The heat load generated by resistive wall wakefields is considered as well. Results are presented for power losses of every element in the 1.3-GHz cryomodule, caused by HOM excitation in the acceleration RF system of the continuous wave linac of SHINE.
keywordPower loss;Higher-order modes (HOMs);Resistive wall wakefields;Impedance;Superconducting cavities;
Research article 05 Jun 2019
Yong-Fang Liu,Zhi-Hao Chen,Hiroshi Matsumoto,Ming Gu,Xiao-Xuan Zhou,Yong-Hua Wu
A C-band accelerator structure was used to accelerate electrons at the Shanghai Soft X-ray Free-Electron Laser Test Facility (SXFEL-TF) in Shanghai Institute of Applied Physics (SINAP). The microwave system of this accelerator structure used a 110 MW pulse modulator and a klystron (PV-5050) to provide the power supply. A pulse transformer is a crucial device in a modulator klystron system, and plays significant roles in voltage level transformation, matching impedances, and polarity inversion. This study presents the optimization of a high-voltage pulse transformer. The design considerations of reducing flattop ringing and flattop droop, and shortening leading edge are provided. The model simulation, mechanical design, and the relevant experimental results are also presented.
keywordPulse transformer;Pulse modulator;Flattop droop;Leading edge;Flattop ringing.;
Research article 12 Jun 2019
Lei Shang,Zhen-Biao Sun,Feng-Lei Shang,Yun-Gai Tang,Wei Liu,Wen-Bin Song
Longitudinal injection is a promising on-axis injection scheme for diffraction-limited storage rings (DLSR). In the latest version of the Hefei Advanced Light Source (HALS), both the dynamic aperture and momentum aperture have been optimized. A longitudinal injection scheme was investigated on the HALS using a double-frequency radio frequency system. To evaluate the injection performance, various errors were considered. A series of tracking simulations were conducted, and the injection efficiency was obtained under different error levels.
keywordInjection efficiency;Longitudinal injection;Hefei Advanced Light Source;Double-frequency RF system;
NUCLEAR ELECTRONICS AND INSTRUMENTATION
Research article 05 Jun 2019
Huai-Qiang Zhang,Zhuo-Dai Li,Bin Tang,He-Xi Wu
CR-RCm filters are widely used in nuclear energy spectrum measurement systems. The choice of parameters of a CR-RCm digital filter directly affects its performance in terms of energy resolution and pulse count rate in digital nuclear spectrometer systems. A numerical recursive model of a CR differential circuit and RC integration circuit is derived, which shows that the shaping result of CR-RCm is determined by the adjustment parameter (k, it determines the shaping time of the shaper) and the integral number (m). Furthermore, the amplitude-frequency response of CR-RCm is analyzed, which shows that it is a bandpass filter; the larger the shaping parameters (k and m), the narrower is the frequency band. CR-RCm digital Gaussian shaping is performed on the actual sampled nuclear pulse signal under different shaping parameters. The energy spectrum of 137Cs is measured based on the LaBr3(Ce) detector under different parameters. The results show that the larger the shaping parameters (m and k), the closer the shaping result is to Gaussian shape, the wider is the shaped pulse, the higher is the energy resolution, and the lower is the pulse count rate. For the same batch of pulse signals, the energy resolution is increased from 3.8% to 3.5%, and the full energy peak area is reduced from 7815 to 6503. Thus, the optimal shaping parameters are m=3 and k=0.95. These research results can provide a design reference for the development of digital nuclear spectrometer measurement systems.
keywordEnergy resolution;Nuclear pulse signal;CR-RCm digital filter;Gaussian shaping;
Research article 11 Jun 2019
Bin Li,Wen-Jing Liu,Ping Zhang,Tong Sun,Lin Li,Yu-Hui Wei,Kai-Zhe Wang,Lin Liu
The arrangement of DNA-based nanostructures into the desired large-scale periodic pattern with the highest possible accuracy and control is essential for the DNA application in functional biomaterials; however, formation of a DNA nanostructure pattern without utilizing the molecular interactions in nanotechnology field remains difficult. In this article, we use the optimal concentration and adsorption time of origami to induce DNA origami in the form of a large-scale 2D pattern on mica without changing the origami itself. DNA origami structures can form a pattern by close-packing of symmetric and electrostatic interactions between ions, which was confirmed by the atomic force microscopy images. Furthermore, we identified favorable conditions for the concentration of DNA origami and optimal adsorption time, which can enable pattern formation with DNA origami. This work provides an insight to understand the adsorption of DNA on mica and guides researches on regular DNA nanostructure pattern, which can serve as templates for pattern formation of proteins or other biomolecules.
keywordDNA;Atomic force microscopy;Origami;Pattern;Close-packing;
NUCLEAR ENERGY SCIENCE AND ENGINEERING
Research article 11 Jun 2019
He Tie,Zheng Pu,Xiao Jun
A measurement of the 235U prompt fission neutron spectrum (PFNS) by the recoil proton method was performed at the Institute of Nuclear Physics and Chemistry (INPC), China. Details of the method, which include the calculation and validation of the response matrix, are presented. The PFNS for 235U in the energy range 1 − 12 MeV, induced by thermal neutrons, was obtained. The measured spectrum in the low-energy region was in good agreement with previous work and the ENDF/B-VII library, except for minor differences. In the high-energy region, however, the relative height of the measured spectrum was greater, and an analysis of the experiment indicated uncertainties of 13% at 10 MeV and 24% at 12 MeV. Experimental results showed that the recoil proton method could be used to measure prompt fission neutron spectra. Some directions for future work are included.
keywordresponse matrix;Prompt fission neutron spectra;Recoil proton method;U-235;
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